دورية أكاديمية
Probing the structure and dynamics of molecular clusters using rotational wave packets.
العنوان: | Probing the structure and dynamics of molecular clusters using rotational wave packets. |
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المؤلفون: | Galinis G; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom., Cacho C; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Chapman RT; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Ellis AM; University of Leicester, Department of Chemistry, Leicester LE1 7RH, United Kingdom., Lewerenz M; Université Paris-Est, Laboratoire Modélisation et Simulation Multi Echelle, MSME UMR 8208 CNRS, 5 bd Descartes, 77454 Marne-la-Vallée, France., Mendoza Luna LG; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom., Minns RS; University of Southampton, Chemistry, Southampton SO17 1BJ, United Kingdom., Mladenović M; Université Paris-Est, Laboratoire Modélisation et Simulation Multi Echelle, MSME UMR 8208 CNRS, 5 bd Descartes, 77454 Marne-la-Vallée, France., Rouzée A; Max Born Institute, Max Born Strasse 2A, 12489 Berlin, Germany., Springate E; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Turcu IC; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Watkins MJ; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom., von Haeften K; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom. |
المصدر: | Physical review letters [Phys Rev Lett] 2014 Jul 25; Vol. 113 (4), pp. 043004. Date of Electronic Publication: 2014 Jul 24. |
نوع المنشور: | Journal Article |
اللغة: | English |
بيانات الدورية: | Publisher: American Physical Society Country of Publication: United States NLM ID: 0401141 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1079-7114 (Electronic) Linking ISSN: 00319007 NLM ISO Abbreviation: Phys Rev Lett Subsets: PubMed not MEDLINE |
أسماء مطبوعة: | Original Publication: New York : American Physical Society |
مستخلص: | Rotational wave packets of the weakly bound C(2)H(2)-He complex have been created using impulsive alignment. The coherent rotational dynamics were monitored for 600 ps enabling extraction of a frequency spectrum showing multiple rotational energy levels up to J = 4. spectrum has been combined with ab initio calculations to show that the complex has a highly delocalized structure and is bound only by ca. 7 cm(-1). The experiments demonstrate how highly featured rotational spectra can be obtained from an extremely cold environment where only the lowest rotational energy states are initially populated. |
تواريخ الأحداث: | Date Created: 20140809 Date Completed: 20150512 Latest Revision: 20140809 |
رمز التحديث: | 20221213 |
DOI: | 10.1103/PhysRevLett.113.043004 |
PMID: | 25105616 |
قاعدة البيانات: | MEDLINE |
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