دورية أكاديمية

Probing the structure and dynamics of molecular clusters using rotational wave packets.

التفاصيل البيبلوغرافية
العنوان: Probing the structure and dynamics of molecular clusters using rotational wave packets.
المؤلفون: Galinis G; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom., Cacho C; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Chapman RT; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Ellis AM; University of Leicester, Department of Chemistry, Leicester LE1 7RH, United Kingdom., Lewerenz M; Université Paris-Est, Laboratoire Modélisation et Simulation Multi Echelle, MSME UMR 8208 CNRS, 5 bd Descartes, 77454 Marne-la-Vallée, France., Mendoza Luna LG; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom., Minns RS; University of Southampton, Chemistry, Southampton SO17 1BJ, United Kingdom., Mladenović M; Université Paris-Est, Laboratoire Modélisation et Simulation Multi Echelle, MSME UMR 8208 CNRS, 5 bd Descartes, 77454 Marne-la-Vallée, France., Rouzée A; Max Born Institute, Max Born Strasse 2A, 12489 Berlin, Germany., Springate E; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Turcu IC; Central Laser Facility, STFC Rutherford Appleton Laboratory, Harwell Oxford, Didcot, Oxfordshire OX11 0QX, United Kingdom., Watkins MJ; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom., von Haeften K; University of Leicester, Department of Physics & Astronomy, Leicester LE1 7RH, United Kingdom.
المصدر: Physical review letters [Phys Rev Lett] 2014 Jul 25; Vol. 113 (4), pp. 043004. Date of Electronic Publication: 2014 Jul 24.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: American Physical Society Country of Publication: United States NLM ID: 0401141 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1079-7114 (Electronic) Linking ISSN: 00319007 NLM ISO Abbreviation: Phys Rev Lett Subsets: PubMed not MEDLINE
أسماء مطبوعة: Original Publication: New York : American Physical Society
مستخلص: Rotational wave packets of the weakly bound C(2)H(2)-He complex have been created using impulsive alignment. The coherent rotational dynamics were monitored for 600 ps enabling extraction of a frequency spectrum showing multiple rotational energy levels up to J = 4. spectrum has been combined with ab initio calculations to show that the complex has a highly delocalized structure and is bound only by ca. 7 cm(-1). The experiments demonstrate how highly featured rotational spectra can be obtained from an extremely cold environment where only the lowest rotational energy states are initially populated.
تواريخ الأحداث: Date Created: 20140809 Date Completed: 20150512 Latest Revision: 20140809
رمز التحديث: 20221213
DOI: 10.1103/PhysRevLett.113.043004
PMID: 25105616
قاعدة البيانات: MEDLINE