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Theoretical study and analysis of o-nitrophenol adsorption using layered double hydroxides containing Ca-Al, Ni-Al and Zn-Al.

التفاصيل البيبلوغرافية
العنوان: Theoretical study and analysis of o-nitrophenol adsorption using layered double hydroxides containing Ca-Al, Ni-Al and Zn-Al.
المؤلفون: Sellaoui L; Department of Environmental Engineering, School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, People's Republic of China. sellaouilotfi@yahoo.fr.; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, 430074, People's Republic of China. sellaouilotfi@yahoo.fr., Yazidi A; Laboratory of Quantum and Statistical Physics, LR18ES18, Faculty of Sciences of Monastir, Monastir University, Monastir, Tunisia., Ali J; Department of Environmental Engineering, School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, People's Republic of China.; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, 430074, People's Republic of China., Dotto GL; Chemical Engineering Department, Federal University of Santa Maria-UFSM, 1000, Roraima Avenue, Santa Maria, RS, 97105-900, Brazil., Bonilla-Petriciolet A; Instituto Tecnológico de Aguascalientes, Aguascalientes, 20256, México., Oliveira LFS; Department of Civil and Environmental, Universidad de la Costa, Calle 58 #55-66, 080002, Barranquilla, Atlantico, Colombia., Badawi M; Laboratoire de Physique et Chimie Théoriques LPCT UMR CNRS 7019, Université de Lorraine, Vandœuvre-lès-Nancy, France., Chen Z; Department of Environmental Engineering, School of Environmental Science and Engineering, Huazhong University of Science and Technology, Wuhan, 430074, People's Republic of China. zqchen@hust.edu.cn.; Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan, 430074, People's Republic of China. zqchen@hust.edu.cn.
المصدر: Environmental science and pollution research international [Environ Sci Pollut Res Int] 2021 Aug; Vol. 28 (32), pp. 44547-44556. Date of Electronic Publication: 2021 Apr 14.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Springer Country of Publication: Germany NLM ID: 9441769 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1614-7499 (Electronic) Linking ISSN: 09441344 NLM ISO Abbreviation: Environ Sci Pollut Res Int Subsets: MEDLINE
أسماء مطبوعة: Publication: <2013->: Berlin : Springer
Original Publication: Landsberg, Germany : Ecomed
مواضيع طبية MeSH: Hydroxides* , Nitrophenols*, Adsorption ; Kinetics ; Models, Theoretical ; Zinc
مستخلص: A theoretical assessment of the o-nitrophenol adsorption on layered double hydroxides containing different metallic species (Ca-Al, Ni-Al and Zn-Al) was performed. Experimental o-nitrophenol adsorption isotherms obtained at different adsorption temperatures with these layered double hydroxides were analyzed using a statistical physics monolayer model. Model calculations showed that the o-nitrophenol aggregation could occur with a high degree. It was estimated that the o-nitrophenol adsorption implied a non-flat orientation on all adsorbent surfaces and this process was multi-molecular. It was also demonstrated that there was no significant difference on the o-nitrophenol adsorption capacities of tested adsorbents, which varied from 77 to 135, 95 to 122 and 74 and 130 mg/g for Ca-Al, Ni-Al and Zn-Al layered double hydroxides, respectively. This finding suggested that the incorporation of Ca-Al, Ni-Al and Zn-Al in the layered double hydroxide structure played a similar role to adsorb o-nitrophenol molecules from aqueous solution. Calculated adsorption energies and thermodynamic functions confirmed an exothermic adsorption with the presence of physical-based interaction forces. This paper highlights the importance of reliable theoretical calculations based on statistical physics theory to contribute in the understanding of the adsorption mechanisms of a relevant water pollutant using layered double hydroxides as promising adsorbents for industrial applications.
(© 2021. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)
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فهرسة مساهمة: Keywords: Layered double hydroxides; Modelling; Multi-molecular adsorption; O-nitrophenol
المشرفين على المادة: 0 (Hydroxides)
0 (Nitrophenols)
J41CSQ7QDS (Zinc)
تواريخ الأحداث: Date Created: 20210415 Date Completed: 20210813 Latest Revision: 20210813
رمز التحديث: 20231215
DOI: 10.1007/s11356-021-13882-x
PMID: 33855661
قاعدة البيانات: MEDLINE
الوصف
تدمد:1614-7499
DOI:10.1007/s11356-021-13882-x