دورية أكاديمية
Cancer risk assessment and source apportionment of the gas- and particulate-phase of the polycyclic aromatic hydrocarbons in a metropolitan region in Brazil.
| العنوان: | Cancer risk assessment and source apportionment of the gas- and particulate-phase of the polycyclic aromatic hydrocarbons in a metropolitan region in Brazil. |
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| المؤلفون: | Galvão ES; Departamento de Engenharia Sanitária e Ambiental, Universidade Federal de Minas Gerais, Belo Horizonte, MG, 31270, Brazil., Paiva HB; Departamento de Química, Universidade Federal de Minas Gerais, Belo Horizonte, MG, 31270, Brazil., Menezes HC; Departamento de Química, Universidade Federal de Minas Gerais, Belo Horizonte, MG, 31270, Brazil., de Almeida Albuquerque TT; Departamento de Engenharia Sanitária e Ambiental, Universidade Federal de Minas Gerais, Belo Horizonte, MG, 31270, Brazil., Cardeal ZL; Departamento de Química, Universidade Federal de Minas Gerais, Belo Horizonte, MG, 31270, Brazil. Electronic address: zenilda@ufmg.br. |
| المصدر: | Chemosphere [Chemosphere] 2023 Jan; Vol. 311 (Pt 1), pp. 136872. Date of Electronic Publication: 2022 Oct 14. |
| نوع المنشور: | Journal Article |
| اللغة: | English |
| بيانات الدورية: | Publisher: Elsevier Science Ltd Country of Publication: England NLM ID: 0320657 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1879-1298 (Electronic) Linking ISSN: 00456535 NLM ISO Abbreviation: Chemosphere Subsets: MEDLINE |
| أسماء مطبوعة: | Publication: Oxford : Elsevier Science Ltd Original Publication: Oxford, New York, : Pergamon Press. |
| مواضيع طبية MeSH: | Polycyclic Aromatic Hydrocarbons*/analysis , Neoplasms* , Air Pollutants*/analysis, Humans ; Gasoline/analysis ; Environmental Monitoring ; Brazil/epidemiology ; Coal/analysis ; Dust/analysis ; Risk Assessment ; Particulate Matter/analysis ; China |
| مستخلص: | A risk assessment and a source apportionment of the particulate- and gas-phase PAHs were conducted in a high vehicular traffic and industrialized region in southeastern Brazil. Higher concentrations of PAHs were found during summer, being likely driven by the contributions of PAHs in the vapor phase caused by fire outbreaks during this period. Isomer ratio diagnostic and Principal Component Analysis (PCA) identified four potential sources in the region, in which the Positive Matrix Factorization (PMF) model confirmed and apportioned as gasoline-related (31.8%), diesel-related (25.1%), biomass burning (23.4%), and mixed sources (19.6%). The overall cancer risk had a tolerable value, with ∑CR = 4.6 × 10 -5 , being ingestion the major via of exposure (64% of the ∑CR), followed by dermal contact (33% of the ∑CR) and inhalation (3%). Mixed sources contributed up to 45% of the overall cancer risk (∑CR), followed by gasoline-related (up to 35%), diesel-related (up to 15%), and biomass burning (up to 10%). The risk assessment for individual PAH species allowed identifying higher CR associated with BaP, DBA, BbF, BaA, and BkF, species associated with gasoline-related and industrial sources. Higher risks were associated with PM Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper. (Copyright © 2022 Elsevier Ltd. All rights reserved.) |
| فهرسة مساهمة: | Keywords: Cancer risk assessment; PAHs; PM(2.5); PMF; Source apportionment |
| المشرفين على المادة: | 0 (Polycyclic Aromatic Hydrocarbons) 0 (Gasoline) 0 (Coal) 0 (Dust) 0 (Air Pollutants) 0 (Particulate Matter) |
| تواريخ الأحداث: | Date Created: 20221017 Date Completed: 20221123 Latest Revision: 20221123 |
| رمز التحديث: | 20231215 |
| DOI: | 10.1016/j.chemosphere.2022.136872 |
| PMID: | 36252898 |
| قاعدة البيانات: | MEDLINE |
Full Text Finder | تدمد: | 1879-1298 |
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| DOI: | 10.1016/j.chemosphere.2022.136872 |