دورية أكاديمية
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Zwitterionic "Solutions" for Reversible CO 2 Capture.

التفاصيل البيبلوغرافية
العنوان: Zwitterionic "Solutions" for Reversible CO 2 Capture.
المؤلفون: Aydos GLP; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Marin G; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Ebeling G; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Dos Santos FP; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Leal BC; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Zink RD; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Vargas BA; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Migowski P; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Stieler R; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., de Araújo BB; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Gonçalves P; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Stassen HK; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil., Dos Santos Pereira L; Petrobras/CENPES, Cidade Universitária, Ilha do Fundão, Avenida Horácio Macedo 950, Rio de Janeiro, RJ, CEP, 21941-915, Brazil., Musse AP; Petrobras/CENPES, Cidade Universitária, Ilha do Fundão, Avenida Horácio Macedo 950, Rio de Janeiro, RJ, CEP, 21941-915, Brazil., Dupont J; Institute of Chemistry, Universidade Federal do Rio Grande do Sul-UFRGS, Av. Bento Gonçalves, 9500, Porto Alegre, 91501-970 RS, Brazil.
المصدر: ChemSusChem [ChemSusChem] 2023 Dec 07; Vol. 16 (23), pp. e202300971. Date of Electronic Publication: 2023 Sep 14.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 101319536 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1864-564X (Electronic) Linking ISSN: 18645631 NLM ISO Abbreviation: ChemSusChem Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Original Publication: Weinheim : Wiley-VCH
مستخلص: The zwitterions resulting from the covalent attachment of 3- or 4-hydroxy benzene to the 1,3-dimethylimidazolium cation represent basic compounds (pKa of 8.68 and 8.99 in aqueous solutions, respectively) that chemisorb in aqueous solutions 0.58 mol/mol of carbon dioxide at 1.3 bar (absolute) and 40 °C. Equimolar amounts of chemisorbed CO 2 in these solutions are obtained at 10 bar and 40 °C. Chemisorption takes place through the formation of bicarbonate in the aqueous solution using imidazolium-containing phenolate. CO 2 is liberated by simple pressure relief and heating, regenerating the base. The enthalpy of absorption was estimated to be -38 kJ/mol, which is about 30 % lower than the enthalpy of industrially employed aqueous solutions of MDEA (estimated at -53 kJ/mol using the same experimental apparatus). The physisorption of CO 2 becomes relevant at higher pressures (>10 bar) in these aqueous solutions. Combined physio- and chemisorption of up to 1.3 mol/mol at 40 bar and 40 °C can be attained with these aqueous zwitterionic solutions that are thermally stable and can be recycled at least 20 times.
(© 2023 Wiley-VCH GmbH.)
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معلومات مُعتمدة: 001 CAPES; 22/2551-0000386-9 FAPERGS; 406260/2018-4 CNPq; SAP4600579154 PETROBRAS
فهرسة مساهمة: Keywords: bicarbonate; carbon dioxide capture; ionic liquids; organic base; zwitterion
تواريخ الأحداث: Date Created: 20230908 Latest Revision: 20231208
رمز التحديث: 20231215
DOI: 10.1002/cssc.202300971
PMID: 37681317
قاعدة البيانات: MEDLINE
الوصف
تدمد:1864-564X
DOI:10.1002/cssc.202300971