دورية أكاديمية

Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents.

التفاصيل البيبلوغرافية
العنوان: Nanofiltration combined with ozone-based processes for the removal of antineoplastic drugs from wastewater effluents.
المؤلفون: Gouveia TIA; LEPABE - Laboratory for Process, Environmental, Biotechnology and Energy Engineering, Faculty of Engineering, University of Porto, R. Dr. Roberto Frias, 4200-465, Porto, Portugal; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal., Gorito AM; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal; CIIMAR/CIMAR - Interdisciplinary Centre of Marine and Environmental Research, Universidade do Porto, Terminal de Cruzeiros do Porto de Leixões, Av. General Norton de Matos, 4450-208, Matosinhos, Portugal; LSRE-LCM - Laboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal., Cristóvão MB; iBET - Instituto de Biologia Experimental e Tecnológica, Apartado 12, 2781-901, Oeiras, Portugal; LAQV- REQUIMTE - Department of Chemistry, NOVA School of Science and Technology, Universidade NOVA de Lisboa, 2829-516, Caparica, Portugal., Pereira VJ; iBET - Instituto de Biologia Experimental e Tecnológica, Apartado 12, 2781-901, Oeiras, Portugal; ITQB NOVA - Instituto de Tecnologia Química e Biológica António Xavier, Universidade Nova de Lisboa, Av. da República, 2780-157, Oeiras, Portugal., Crespo J; LAQV- REQUIMTE - Department of Chemistry, NOVA School of Science and Technology, Universidade NOVA de Lisboa, 2829-516, Caparica, Portugal., Alves A; LEPABE - Laboratory for Process, Environmental, Biotechnology and Energy Engineering, Faculty of Engineering, University of Porto, R. Dr. Roberto Frias, 4200-465, Porto, Portugal; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal., Pereira MFR; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal; LSRE-LCM - Laboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal., Ribeiro ARL; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal; LSRE-LCM - Laboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal., Silva AMT; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal; LSRE-LCM - Laboratory of Separation and Reaction Engineering - Laboratory of Catalysis and Materials, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal. Electronic address: adrian@fe.up.pt., Santos MSF; LEPABE - Laboratory for Process, Environmental, Biotechnology and Energy Engineering, Faculty of Engineering, University of Porto, R. Dr. Roberto Frias, 4200-465, Porto, Portugal; ALiCE - Associate Laboratory in Chemical Engineering, Faculty of Engineering, University of Porto, Rua Dr. Roberto Frias, 4200-465, Porto, Portugal; EPIUnit - Institute of Public Health, University of Porto, Rua das Taipas, n° 135, 4050-600, Porto, Portugal; Laboratory for Integrative and Translational Research in Population Health (ITR), University of Porto, Rua das Taipas, n° 135, 4050-600, Porto, Portugal. Electronic address: monica.santos@ispup.up.pt.
المصدر: Journal of environmental management [J Environ Manage] 2023 Dec 15; Vol. 348, pp. 119314. Date of Electronic Publication: 2023 Oct 17.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Academic Press Country of Publication: England NLM ID: 0401664 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1095-8630 (Electronic) Linking ISSN: 03014797 NLM ISO Abbreviation: J Environ Manage Subsets: MEDLINE
أسماء مطبوعة: Original Publication: London ; New York, Academic Press.
مواضيع طبية MeSH: Drinking Water* , Ozone* , Water Pollutants, Chemical*/analysis , Water Purification*/methods , Antineoplastic Agents*, Wastewater ; Hydrogen Peroxide ; Pharmaceutical Preparations ; Oxidation-Reduction
مستخلص: Over the past years, there has been an increasing concern about the occurrence of antineoplastic drugs in water bodies. The incomplete removal of these pharmaceuticals from wastewaters has been confirmed by several scientists, making it urgent to find a reliable technique or a combination of techniques capable to produce clean and safe water. In this work, the combination of nanofiltration and ozone (O 3 )-based processes (NF + O 3 , NF + O 3 /H 2 O 2 and NF + O 3 /H 2 O 2 /UVA) was studied aiming to produce clean water from wastewater treatment plant (WWTP) secondary effluents to be safely discharged into water bodies, reused in daily practices such as aquaculture activities or for recharging aquifers used as abstraction sources for drinking water production. Nanofiltration was performed in a pilot-scale unit and O 3 -based processes in a continuous-flow column. The peroxone process (O 3 /H 2 O 2 ) was considered the most promising technology to be coupled to nanofiltration, all the target pharmaceuticals being removed at an extent higher than 98% from WWTP secondary effluents, with a DOC reduction up to 92%. The applicability of the clean water stream for recharging aquifers used as abstraction sources for drinking water production was supported by a risk assessment approach, regarding the final concentrations of the target pharmaceuticals. Moreover, the toxicity of the nanofiltration retentate, a polluted stream generated from the nanofiltration system, was greatly decreased after the application of the peroxone process, which evidences the positive impact on the environment of implementing a NF + O 3 /H 2 O 2 process.
Competing Interests: Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
(Copyright © 2023 The Authors. Published by Elsevier Ltd.. All rights reserved.)
فهرسة مساهمة: Keywords: Anticancer drugs; Cytostatics; Nanofiltration; Ozonation; Peroxone; Risk assessment; Wastewater effluent
المشرفين على المادة: 0 (Wastewater)
BBX060AN9V (Hydrogen Peroxide)
0 (Drinking Water)
66H7ZZK23N (Ozone)
0 (Water Pollutants, Chemical)
0 (Antineoplastic Agents)
0 (Pharmaceutical Preparations)
تواريخ الأحداث: Date Created: 20231019 Date Completed: 20231115 Latest Revision: 20231115
رمز التحديث: 20240628
DOI: 10.1016/j.jenvman.2023.119314
PMID: 37857217
قاعدة البيانات: MEDLINE
الوصف
تدمد:1095-8630
DOI:10.1016/j.jenvman.2023.119314