دورية أكاديمية
Self-Propulsion by Directed Explosive Emulsification.
| العنوان: | Self-Propulsion by Directed Explosive Emulsification. |
|---|---|
| المؤلفون: | Wu X; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA., Xue H; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA., Bordia G; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.; Department of Materials Science and Engineering, University of California Berkeley, Berkeley, CA, 94720, USA., Fink Z; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.; Polymer Science and Engineering Department, University of Massachusetts, Amherst, MA, 01003, USA., Kim PY; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA., Streubel R; Department of Physics and Astronomy, University of Nebraska-Lincoln, Lincoln, NE, 68588, USA., Han J; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.; Department of Materials Science and Engineering, University of California Berkeley, Berkeley, CA, 94720, USA., Helms BA; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.; Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA., Ashby PD; Molecular Foundry, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA., Omar AK; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.; Department of Materials Science and Engineering, University of California Berkeley, Berkeley, CA, 94720, USA., Russell TP; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA, 94720, USA.; Polymer Science and Engineering Department, University of Massachusetts, Amherst, MA, 01003, USA. |
| المصدر: | Advanced materials (Deerfield Beach, Fla.) [Adv Mater] 2024 May; Vol. 36 (19), pp. e2310435. Date of Electronic Publication: 2024 Feb 29. |
| نوع المنشور: | Journal Article |
| اللغة: | English |
| بيانات الدورية: | Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 9885358 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-4095 (Electronic) Linking ISSN: 09359648 NLM ISO Abbreviation: Adv Mater Subsets: PubMed not MEDLINE; MEDLINE |
| أسماء مطبوعة: | Publication: Sept. 3, 1997- : Weinheim : Wiley-VCH Original Publication: Deerfield Beach, FL : VCH Publishers, 1989- |
| مستخلص: | An active droplet system, programmed to repeatedly move autonomously at a specific velocity in a well-defined direction, is demonstrated. Coulombic energy is stored in oversaturated interfacial assemblies of charged nanoparticle-surfactants by an applied DC electric field and can be released on demand. Spontaneous emulsification is suppressed by an increase in the stiffness of the oversaturated assemblies. Rapidly removing the field releases the stored energy in an explosive event that propels the droplet, where thousands of charged microdroplets are ballistically ejected from the surface of the parent droplet. The ejection is made directional by a symmetry breaking of the interfacial assembly, and the combined interaction force of the microdroplet plume on one side of the droplet propels the droplet distances tens of times its size, making the droplet active. The propulsion is autonomous, repeatable, and agnostic to the chemical composition of the nanoparticles. The symmetry-breaking in the nanoparticle assembly controls the microdroplet velocity and direction of propulsion. This mechanism of droplet propulsion will advance soft micro-robotics, establishes a new type of active matter, and introduces new vehicles for compartmentalized delivery. (© 2024 Wiley‐VCH GmbH.) |
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| معلومات مُعتمدة: | U.S. Department of Energy; Office of Science; Basic Energy Sciences; DE-AC02-05-CH11231 Materials Sciences and Engineering Division; KCTR16 Adaptive Interfacial Assemblies Towards Structuring Liquids program; DE-AC02-05CH11231 Division of Materials Research; 2203933 National Science Foundation |
| فهرسة مساهمة: | Keywords: charged nanoparticle‐surfactants; directed explosive emulsification; liquid–liquid interface; self‐assembly; self‐propulsion |
| تواريخ الأحداث: | Date Created: 20240222 Latest Revision: 20240509 |
| رمز التحديث: | 20240510 |
| DOI: | 10.1002/adma.202310435 |
| PMID: | 38386499 |
| قاعدة البيانات: | MEDLINE |
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