دورية أكاديمية
Effect of Salts on Laccase-Catalyzed Polymerization of Lignosulfonate.
| العنوان: | Effect of Salts on Laccase-Catalyzed Polymerization of Lignosulfonate. |
|---|---|
| المؤلفون: | Mayr SA; University of Natural Resources and Life Sciences, Vienna, Department of Agrobiotechnology, IFA-Tulln, Institute of Environmental Biotechnology, Konrad Lorenz-Strasse 20, 3430, Tulln an der Donau, Austria., Rennhofer H; University of Natural Resources and Life Sciences, Vienna, Department of Material Science and Process Engineering, Institute of Physics and Material Science, Peter-Jordan-Strasse 82, 1190, Vienna, Austria., Gille L; University of Veterinary Medicine, Vienna, Department of Biomedical Sciences, Institute of Pharmacology and Toxicology, Veterinärplatz 1, 1210, Vienna, Austria., Schwaiger N; Sappi paper holding GmbH, Brucker Strasse 21, 8101, Gratkorn, Austria., Nyanhongo GS; University of Johannesburg, Department of Biotechnology and Food Technology, Faculty of Science, Corner Siemert and Louisa, Doornfontein 2028, John Orr Building, Johannesburg, South Africa., Weiss R; University of Natural Resources and Life Sciences, Vienna, Department of Agrobiotechnology, IFA-Tulln, Institute of Environmental Biotechnology, Konrad Lorenz-Strasse 20, 3430, Tulln an der Donau, Austria., Guebitz GM; University of Natural Resources and Life Sciences, Vienna, Department of Agrobiotechnology, IFA-Tulln, Institute of Environmental Biotechnology, Konrad Lorenz-Strasse 20, 3430, Tulln an der Donau, Austria.; Austrian Centre for Industrial Biotechnology (ACIB), Konrad Lorenz Strasse 20, 3430, Tulln, Austria. |
| المصدر: | ChemSusChem [ChemSusChem] 2024 Mar 08, pp. e202301134. Date of Electronic Publication: 2024 Mar 08. |
| Publication Model: | Ahead of Print |
| نوع المنشور: | Journal Article |
| اللغة: | English |
| بيانات الدورية: | Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 101319536 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1864-564X (Electronic) Linking ISSN: 18645631 NLM ISO Abbreviation: ChemSusChem Subsets: MEDLINE |
| أسماء مطبوعة: | Original Publication: Weinheim : Wiley-VCH |
| مستخلص: | Enzymatic polymerization of lignosulfonate (LS) has a high potential for various applications ranging from coatings to adhesives. Here, the effect of different ions in low concentrations on enzymatic polymerization of LS was investigated, including salt solutions consisting of mono- and dicarboxylic acids, sulfate, phosphate and chloride with sodium as counter ion. LS polymerization was followed by viscometry and size exclusion (SEC) chromatography. Interestingly, there was only a small effect of ions on the activity of the laccase on standard substrate ABTS, while the effect on polymerization of LS was substantially different. The presence of acetate led to a 39 % higher degree of polymerization (DP) for LS. Small angle X-ray scattering (SAXS) revealed that the structure of the enzyme was largely unaffected by the ions, while the determination of the zeta potential showed that those ions conveying higher negative surface charges onto LS particles showed lower DPs, than those not affecting the surface charge. Further, electron paramagnetic resonance (EPR) spectroscopy showed 5-times higher intensity in phenoxyl radicals for the monovalent ions compared to the divalent ones. It was concluded that the DPs of LS could be tuned in the presence of certain ions, by facilitating the interaction between the laccase substrate-binding site and the LS molecules. (© 2024 The Authors. ChemSusChem published by Wiley-VCH GmbH.) |
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| معلومات مُعتمدة: | 792021 Biobased Industries Joint Undertaking (BBI-JU) |
| فهرسة مساهمة: | Keywords: anions; green chemistry; laccase; oxidation; radical reactions |
| تواريخ الأحداث: | Date Created: 20240308 Latest Revision: 20240418 |
| رمز التحديث: | 20240418 |
| DOI: | 10.1002/cssc.202301134 |
| PMID: | 38456224 |
| قاعدة البيانات: | MEDLINE |
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