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A correlated ferromagnetic polar metal by design.

التفاصيل البيبلوغرافية
العنوان: A correlated ferromagnetic polar metal by design.
المؤلفون: Zhang J; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China., Shen S; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China., Puggioni D; Department of Materials Science and Engineering, Northwestern University, Evanston, IL, USA., Wang M; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China., Sha H; State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China.; MOE Key Laboratory of Advanced Materials, Tsinghua University, Beijing, China., Xu X; High Magnetic Field Laboratory, HFIPS, Anhui, Chinese Academy of Sciences, Hefei, China., Lyu Y; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China., Peng H; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China., Xing W; State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China.; MOE Key Laboratory of Advanced Materials, Tsinghua University, Beijing, China., Walters LN; Department of Materials Science and Engineering, Northwestern University, Evanston, IL, USA., Liu L; State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China.; MOE Key Laboratory of Advanced Materials, Tsinghua University, Beijing, China., Wang Y; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China., Hou; High Magnetic Field Laboratory, HFIPS, Anhui, Chinese Academy of Sciences, Hefei, China., Xi C; High Magnetic Field Laboratory, HFIPS, Anhui, Chinese Academy of Sciences, Hefei, China., Pi L; High Magnetic Field Laboratory, HFIPS, Anhui, Chinese Academy of Sciences, Hefei, China., Ishizuka H; Department of Physics, Tokyo Institute of Technology, Tokyo, Japan., Kotani Y; Center for Synchrotron Radiation Research, Japan Synchrotron Radiation Research Institute, Hyogo, Japan., Kimata M; Institute of Materials Research, Tohoku University, Sendai, Japan., Nojiri H; Institute of Materials Research, Tohoku University, Sendai, Japan., Nakamura T; International Center for Synchrotron Radiation Innovation Smart, Tohoku University, Sendai, Japan., Liang T; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China.; RIKEN Center for Emergent Matter Science (CEMS), Wako, Japan.; Frontier Science Center for Quantum Information, Beijing, China., Yi D; State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China., Nan T; School of Integrated Circuits, Beijing National Research Center for Information Science and Technology, Tsinghua University, Beijing, China., Zang J; Department of Physics and Astronomy, University of New Hampshire, Durham, NH, USA., Sheng Z; High Magnetic Field Laboratory, HFIPS, Anhui, Chinese Academy of Sciences, Hefei, China., He Q; Department of Physics, Durham University, Durham, UK., Zhou S; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China.; Frontier Science Center for Quantum Information, Beijing, China., Nagaosa N; RIKEN Center for Emergent Matter Science (CEMS), Wako, Japan.; Department of Applied Physics, University of Tokyo, Tokyo, Japan., Nan CW; State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China., Tokura Y; RIKEN Center for Emergent Matter Science (CEMS), Wako, Japan.; Department of Applied Physics, University of Tokyo, Tokyo, Japan., Yu R; State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing, China. ryu@tsinghua.edu.cn.; MOE Key Laboratory of Advanced Materials, Tsinghua University, Beijing, China. ryu@tsinghua.edu.cn., Rondinelli JM; Department of Materials Science and Engineering, Northwestern University, Evanston, IL, USA. jrondinelli@northwestern.edu., Yu P; State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics, Tsinghua University, Beijing, China. yupu@tsinghua.edu.cn.; RIKEN Center for Emergent Matter Science (CEMS), Wako, Japan. yupu@tsinghua.edu.cn.; Frontier Science Center for Quantum Information, Beijing, China. yupu@tsinghua.edu.cn.
المصدر: Nature materials [Nat Mater] 2024 Jul; Vol. 23 (7), pp. 912-919. Date of Electronic Publication: 2024 Apr 11.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Nature Pub. Group Country of Publication: England NLM ID: 101155473 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1476-4660 (Electronic) Linking ISSN: 14761122 NLM ISO Abbreviation: Nat Mater Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Original Publication: London, UK : Nature Pub. Group, [2002]-
مستخلص: Polar metals have recently garnered increasing interest because of their promising functionalities. Here we report the experimental realization of an intrinsic coexisting ferromagnetism, polar distortion and metallicity in quasi-two-dimensional Ca 3 Co 3 O 8 . This material crystallizes with alternating stacking of oxygen tetrahedral CoO 4 monolayers and octahedral CoO 6 bilayers. The ferromagnetic metallic state is confined within the quasi-two-dimensional CoO 6 layers, and the broken inversion symmetry arises simultaneously from the Co displacements. The breaking of both spatial-inversion and time-reversal symmetries, along with their strong coupling, gives rise to an intrinsic magnetochiral anisotropy with exotic magnetic field-free non-reciprocal electrical resistivity. An extraordinarily robust topological Hall effect persists over a broad temperature-magnetic field phase space, arising from dipole-induced Rashba spin-orbit coupling. Our work not only provides a rich platform to explore the coupling between polarity and magnetism in a metallic system, with extensive potential applications, but also defines a novel design strategy to access exotic correlated electronic states.
(© 2024. The Author(s), under exclusive licence to Springer Nature Limited.)
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معلومات مُعتمدة: 2021YFE0107900 National Natural Science Foundation of China (National Science Foundation of China); 2023YFA1406400 National Natural Science Foundation of China (National Science Foundation of China); 2021YFA1400300 National Natural Science Foundation of China (National Science Foundation of China); 52388201 National Natural Science Foundation of China (National Science Foundation of China); Z200007 Natural Science Foundation of Beijing Municipality (Beijing Natural Science Foundation); W911NF-15-1-0017 United States Department of Defense | United States Army | U.S. Army Research, Development and Engineering Command | Army Research Office (ARO); DMR-2104397 National Science Foundation (NSF)
تواريخ الأحداث: Date Created: 20240411 Latest Revision: 20240708
رمز التحديث: 20240709
DOI: 10.1038/s41563-024-01856-6
PMID: 38605196
قاعدة البيانات: MEDLINE
الوصف
تدمد:1476-4660
DOI:10.1038/s41563-024-01856-6