Low-energy formate production from CO2 electroreduction using electrodeposited tin on GDE
العنوان: | Low-energy formate production from CO2 electroreduction using electrodeposited tin on GDE |
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المؤلفون: | Germán Penelas-Pérez, María D. Hernández-Alonso, Erdem Irtem, Teresa Andreu, J. M. Riesco-García, S. García-Rodríguez, Andrés Parra, J. R. Morante |
المصدر: | Journal of Materials Chemistry A. 4:13582-13588 |
بيانات النشر: | Royal Society of Chemistry (RSC), 2016. |
سنة النشر: | 2016 |
مصطلحات موضوعية: | Renewable Energy, Sustainability and the Environment, Formic acid, Inorganic chemistry, chemistry.chemical_element, 02 engineering and technology, General Chemistry, 010402 general chemistry, 021001 nanoscience & nanotechnology, Electrochemistry, 01 natural sciences, 0104 chemical sciences, Catalysis, chemistry.chemical_compound, chemistry, Yield (chemistry), Electrode, General Materials Science, Formate, 0210 nano-technology, Tin, Faraday efficiency |
الوصف: | Tin electrodeposition on carbon fibers have been implemented for gas diffusion electrodes for the electroreduction of CO2 to formate in a electrochemical flow cell design. Unlike other approaches, this method does not incorporate any additive or binder in the electrode, thus improving their catalytic performances. Once optimized, the system shows an improved dependence of the effective production of formate yield by surface and time units, mol m−2 s−1, on the consumed energy by mol, W h mol−1. It reduces the formic acid production energy cost, requiring less than 250 W h mol−1, with formate faradaic efficiency as high as 71% and is fully stable for at least 6 hours. |
تدمد: | 2050-7496 2050-7488 |
URL الوصول: | https://explore.openaire.eu/search/publication?articleId=doi_________::b068940149509485ad1bc4f4f981bfb6 https://doi.org/10.1039/c6ta04432h |
حقوق: | OPEN |
رقم الأكسشن: | edsair.doi...........b068940149509485ad1bc4f4f981bfb6 |
قاعدة البيانات: | OpenAIRE |
تدمد: | 20507496 20507488 |
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