تقرير
Actinide and Lanthanide Dioxide Lattice Dilatation Mechanisms with Defect Ingrowth
| العنوان: | Actinide and Lanthanide Dioxide Lattice Dilatation Mechanisms with Defect Ingrowth |
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| المؤلفون: | Günay, S. D. |
| سنة النشر: | 2020 |
| المجموعة: | Condensed Matter |
| مصطلحات موضوعية: | Condensed Matter - Materials Science |
| الوصف: | {\alpha}-particle irradiated single-crystal isostructural oxide lattices (CmO2, AmO2, CeO2, UO2, NpO2, PuO2, ThO2) were modeled by molecular dynamics simulation method. Lattice parameter changes with IFP cation defects displayed exponential increases. These data were compatible with the available lattice parameter changes with {\alpha}-particle dose experiments. Pre- and post- peaks emerged around principal peaks of irradiated oxide cation-cation radial distribution functions, which indicate obstruction and distortion type defects, respectively. Dependence of lattice dilatations on the number of obstruction type cation defects was examined. In a previous study, obstruction type uranium defects were found to be directly responsible for the UO2 lattice swelling and there was a linear relationship between them. It was also determined that this linear equation has two different slopes at low and high defect concentrations. In this paper, it was found that these phenomena were not specific to UO2 and applicable to all fluorite-structured actinide and lanthanide dioxides studied here. These findings provide clues about the existence of more general law. Comment: 44 pages, 8 Figures, 4 Tables, Supplementary Material |
| نوع الوثيقة: | Working Paper |
| DOI: | 10.1111/jace.19020 |
| URL الوصول: | http://arxiv.org/abs/2002.00574 |
| رقم الأكسشن: | edsarx.2002.00574 |
| قاعدة البيانات: | arXiv |
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