تقرير
Tetragonal mixed system $Cs_2CuCl_{4-x}Br_x$ complemented by the tetragonal phase realisation of $Cs_2CuCl_4$
| العنوان: | Tetragonal mixed system $Cs_2CuCl_{4-x}Br_x$ complemented by the tetragonal phase realisation of $Cs_2CuCl_4$ |
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| المؤلفون: | van Well, Natalija, Eisele, Claudio, Ramakrishnan, Sitaram, Shang, Tian, Medarde, Marisa, Cervellino, Antonio, Skoulatos, Markos, Georgii, Robert, van Smaalen, Sander |
| المصدر: | Cryst. Growth Des. 2019, 19, 6627-6635 |
| سنة النشر: | 2020 |
| المجموعة: | Condensed Matter |
| مصطلحات موضوعية: | Condensed Matter - Materials Science, Condensed Matter - Strongly Correlated Electrons |
| الوصف: | Realisation of the tetragonal phase of $Cs_2CuCl_4$ is possible using specific crystal growth conditions at a temperature below $281K$. This work deals with the comparison of the magnetic susceptibility and the magnetization of this new tetragonal compound with the magnetic behaviour of tetragonal $Cs_2CuCl_{2.9}Br_{1.1}$, $Cs_2CuCl_{2.5}Br_{1.5}$, $Cs_2CuCl_{2.2}Br_{1.8}$ and presents consistent results for such quasi $2-D$ antiferromagnets. Structural investigation at low temperature for $Cs_2CuCl_{2.2}Br_{1.8}$ shows no phase transition. The structure remains in the tetragonal symmetry $I4/mmm$. Furthermore, several magnetic reflections corresponding to the propagation vector $k = (0, 0, 0)$ are observed for this tetragonal compound through neutron diffraction experiments below the magnetic phase transition at $T_N = 11.3K$ confirming its antiferromagnetic nature. Comment: Preprint |
| نوع الوثيقة: | Working Paper |
| DOI: | 10.1021/acs.cgd.9b01035 |
| URL الوصول: | http://arxiv.org/abs/2002.11202 |
| رقم الأكسشن: | edsarx.2002.11202 |
| قاعدة البيانات: | arXiv |
| DOI: | 10.1021/acs.cgd.9b01035 |
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