تقرير
Double photoionization of propylene oxide: a coincidence study of the ejection of a pair of valence-shell electrons
العنوان: | Double photoionization of propylene oxide: a coincidence study of the ejection of a pair of valence-shell electrons |
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المؤلفون: | Falcinelli, Stefano, Vecchiocattivi, Franco, Alagia, Michele, Schio, Luca, Richter, Robert, Stranges, Stefano, Catone, Daniele, Arruda, Manuela S., Mendes, Luiz A. V., Palazzetti, Federico, Aquilanti, Vincenzo, Pirani, Fernando |
سنة النشر: | 2020 |
المجموعة: | Physics (Other) |
مصطلحات موضوعية: | Physics - Atomic Physics |
الوصف: | Propylene oxide, a favorite target of experimental and theoretical studies of circular dichroism, was recently discovered in interstellar space, further amplifying the attention to its role in the current debate on protobiological homochirality. In the present work, a photoelectron-photoion-photoion coincidence technique, using an ion-imaging detector and tunable synchrotron radiation in the 18.0-37.0 eV energy range, permits: (i)-to observe six double-ionization fragmentation channels, their relative yields being accounted for about two-thirds by the couple (C2H4+, CH2O+), one-fifth by (C2H3+, CH3O+); (ii)-to measure thresholds for their openings as a function of photon energy; (iii)-to unravel a pronounced bimodality for a kinetic-energy-released distribution, fingerprint of competitive non-adiabatic mechanisms. Comment: 27 pages, 6 figures |
نوع الوثيقة: | Working Paper |
DOI: | 10.1063/1.5024408 |
URL الوصول: | http://arxiv.org/abs/2004.04639 |
رقم الأكسشن: | edsarx.2004.04639 |
قاعدة البيانات: | arXiv |
DOI: | 10.1063/1.5024408 |
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