Magnetic anisotropy and exchange paths for octa- and tetrahedrally coordinated Mn$^{2+}$ ions in the honeycomb multiferroic Mn$_2$Mo$_3$O$_8$

التفاصيل البيبلوغرافية
العنوان: Magnetic anisotropy and exchange paths for octa- and tetrahedrally coordinated Mn$^{2+}$ ions in the honeycomb multiferroic Mn$_2$Mo$_3$O$_8$
المؤلفون: Szaller, D., Szász, K., Bordács, S., Viirok, J., Rõõm, T., Nagel, U., Shuvaev, A., Weymann, L., Pimenov, A., Tsirlin, A. A., Jesche, A., Prodan, L., Tsurkan, V., Kézsmárki, I.
سنة النشر: 2020
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science
الوصف: We investigated the static and dynamic magnetic properties of the polar ferrimagnet Mn$_2$Mo$_3$O$_8$ in three magnetically ordered phases via magnetization, magnetic torque, and THz absorption spectroscopy measurements. The observed magnetic field dependence of the spin-wave resonances, including Brillouin zone-center and zone-boundary excitations, magnetization, and torque, are well described by an extended two-sublattice antiferromagnetic classical mean-field model. In this orbitally quenched system, the competing weak easy-plane and easy-axis single-ion anisotropies of the two crystallographic sites are determined from the model and assigned to the tetra- and octahedral sites, respectively, by ab initio calculations.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.102.144410
URL الوصول: http://arxiv.org/abs/2009.11683
رقم الأكسشن: edsarx.2009.11683
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.102.144410