Direct visualization and control of antiferromagnetic domains and spin reorientation in a parent cuprate

التفاصيل البيبلوغرافية
العنوان: Direct visualization and control of antiferromagnetic domains and spin reorientation in a parent cuprate
المؤلفون: Seyler, K. L., Ron, A., Van Beveren, D., Rotundu, C. R., Lee, Y. S., Hsieh, D.
المصدر: Phys. Rev. B 106, L140403 (2022)
سنة النشر: 2022
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Superconductivity
الوصف: We report magnetic optical second-harmonic generation (SHG) polarimetry and imaging on Sr$_2$Cu$_3$O$_4$Cl$_2$, which allows direct visualization of the mesoscopic antiferromagnetic (AFM) structure of a parent cuprate. Temperature- and magnetic-field-dependent SHG reveals large domains with 90$^{\circ}$ relative orientations that are stabilized by a combination of uniaxial magnetic anisotropy and the Earth's magnetic field. Below a temperature $T_R$ $\sim$ 97 K, we observe an unusual 90$^{\circ}$ spin reorientation transition, possibly driven by competing magnetic anisotropies of the two copper sublattices, which swaps the AFM domain states while preserving the domain structure. This allows deterministic switching of the AFM states by thermal or laser heating. Near $T_R$, the domain walls become exceptionally responsive to an applied magnetic field, with the Earth's field sufficient to completely expel them from the crystal. Our findings unlock opportunities to study the mesoscopic AFM behavior of parent cuprates and explore their potential for AFM technologies.
Comment: 7 pages main text, 4 figures, 13 pages supplementary information
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.106.L140403
URL الوصول: http://arxiv.org/abs/2210.04327
رقم الأكسشن: edsarx.2210.04327
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.106.L140403