تقرير
Kinetically limited valence of colloidal particles with surface mobile DNA linkers
العنوان: | Kinetically limited valence of colloidal particles with surface mobile DNA linkers |
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المؤلفون: | Sánchez, Pedro A., Caciagli, Alessio, Kantorovich, Sofia S., Eiser, Erika |
سنة النشر: | 2022 |
المجموعة: | Condensed Matter Physics (Other) |
مصطلحات موضوعية: | Condensed Matter - Soft Condensed Matter, Condensed Matter - Mesoscale and Nanoscale Physics, Condensed Matter - Materials Science, Physics - Chemical Physics |
الوصف: | We characterize the self-assembly of colloidal particles with surface mobile DNA linkers under kinetically limited valence conditions. For this, we put forward a computer simulation model that captures quantitatively the interplay between the main dynamic processes governing these systems and allows the simulation of the long time scales reached in experiments. The model is validated by direct comparison with available experimental results, showing an overall good agreement that includes measurements of the average effective valence and its probability distribution as a function of the density of DNA linkers on the particles surface. Finally, simulation results are used to evidence the opposite impact of particle density and characteristic DNA hybridization time on the effective valence. Comment: 10 pages, 6 figures |
نوع الوثيقة: | Working Paper |
URL الوصول: | http://arxiv.org/abs/2210.14209 |
رقم الأكسشن: | edsarx.2210.14209 |
قاعدة البيانات: | arXiv |
الوصف غير متاح. |