Optical absorption of angulon in metal halide perovskites

التفاصيل البيبلوغرافية
العنوان: Optical absorption of angulon in metal halide perovskites
المؤلفون: Wu, Jia-Wei, Cui, Yu, Li, Shao-Juan, Wang, Zi-Wu
سنة النشر: 2022
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics, Condensed Matter - Materials Science
الوصف: We theoretically study the optical absorption of an angulon in the metal halide perovskites (MHP) based on the improved Devreese-Huybrechts-Lemmens model, where the formation of quasiparticle angulon states originates from the organic cation rotating in the inorganic octahedral cage of MHP. We find that the resonance optical absorption peaks are appeared when the energy of incident photon matches the quantum levels of angulon. Moreover, the intensity of absorption depends on the quantum states of phonon angular momentum. These theoretical results provide significant insight to study the redistribution of angular momenta for the rotational molecules immersed into the many-body environment.
Comment: 10 pages, 2 figures
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/2212.06356
رقم الأكسشن: edsarx.2212.06356
قاعدة البيانات: arXiv