Identifying f-electron symmetries of UTe2 with O-edge resonant inelastic X-ray scattering

التفاصيل البيبلوغرافية
العنوان: Identifying f-electron symmetries of UTe2 with O-edge resonant inelastic X-ray scattering
المؤلفون: Liu, Shouzheng, Xu, Yishuai, Kotta, Erica C., Miao, Lin, Ran, Sheng, Paglione, Johnpierre, Butch, Nicholas P., Denlinger, Jonathan D., Chuang, Yi-De, Wray, L. Andrew
المصدر: Phys. Rev. B 106, L241111 (2022)
سنة النشر: 2023
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons
الوصف: The recent discovery of spin-triplet superconductivity emerging from a non-magnetic parent state in UTe$_2$ has stimulated great interest in the underlying mechanism of Cooper pairing. Experimental characterization of short-range electronic and magnetic correlations is vital to understanding these phenomena. Here we use resonant inelastic X-ray scattering (RIXS), X-ray absorption spectroscopy (XAS), and atomic multiplet-based modeling to shed light on the active debate between 5$f^2$6$d^1$-based models with singlet crystal field states versus 5$f^3$-based models that predict atomic Kramers doublets and much greater 5$f$ itinerancy. The XAS and RIXS data are found to agree strongly with predictions for an 5$f^2$6$d^1$-like valence electron configuration with weak intra-dimer magnetic correlations, and provide new context for interpreting recent investigations of the electronic structure and superconducting pairing mechanism.
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevB.106.L241111
URL الوصول: http://arxiv.org/abs/2302.02010
رقم الأكسشن: edsarx.2302.02010
قاعدة البيانات: arXiv
الوصف
DOI:10.1103/PhysRevB.106.L241111