Magnetostriction-Driven Muon Localization in an Antiferromagnetic Oxide

التفاصيل البيبلوغرافية
العنوان: Magnetostriction-Driven Muon Localization in an Antiferromagnetic Oxide
المؤلفون: Bonfà, Pietro, Onuorah, Ifeanyi John, Lang, Franz, Timrov, Iurii, Monacelli, Lorenzo, Wang, Chennan, Sun, Xiao, Petracic, Oleg, Pizzi, Giovanni, Marzari, Nicola, Blundell, Stephen J., De Renzi, Roberto
المصدر: Phys. Rev. Lett. 132, 046701 (2024)
سنة النشر: 2023
المجموعة: Condensed Matter
مصطلحات موضوعية: Condensed Matter - Strongly Correlated Electrons, Condensed Matter - Materials Science
الوصف: Magnetostriction drives a rhombohedral distortion in the cubic rock salt antiferromagnet MnO at the N\'eel temperature $T_{N}=118$ K. As an unexpected consequence we show that this distortion acts to localize the site of an implanted muon due to the accompanying redistribution of electron density. This lifts the degeneracy between equivalent sites, resulting in a single observed muon precession frequency. Above $T_{N}$, the muon instead becomes delocalized around a network of equivalent sites. Our first-principles simulations based on Hubbard-corrected density-functional theory and molecular dynamics are consistent with our experimental data and help to resolve a long-standing puzzle regarding muon data on MnO, as well as having wider applicability to other magnetic oxides.
Comment: 7 pages, 3 figures
نوع الوثيقة: Working Paper
DOI: 10.1103/PhysRevLett.132.046701
URL الوصول: http://arxiv.org/abs/2305.12237
رقم الأكسشن: edsarx.2305.12237
قاعدة البيانات: arXiv