Engineering the directionality of hot carrier tunneling in plasmonic tunneling structures

التفاصيل البيبلوغرافية
العنوان: Engineering the directionality of hot carrier tunneling in plasmonic tunneling structures
المؤلفون: Abbasi, Mahdiyeh, Liao, Shusen, Zhu, Yunxuan, Natelson, Douglas
المصدر: Appl. Phys. Lett. 122, 231103 (2023)
سنة النشر: 2023
المجموعة: Condensed Matter
Physics (Other)
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics, Physics - Optics
الوصف: Tunneling metal-insulator-metal (MIM) junctions can exhibit an open-circuit photovoltage (OCPV) response under illumination that may be useful for photodetection. One mechanism for photovoltage generation is hot carrier tunneling, in which photoexcited carriers generate a net photocurrent that must be balanced by a drift current in the open-circuit configuration. We present experiments in electromigrated planar MIM structures, designed with asymmetric plasmonic properties using Au and Pt electrodes. Decay of optically excited local plasmonic modes preferentially creates hot carriers on the Au side of the junction, leading to a clear preferred directionality of the hot electron photocurrent and hence a preferred polarity of the resulting OCPV. In contrast, in an ensemble of symmetric devices constructed from only one Au, polarity of the OCPV has no preferred direction.
Comment: 17 pages, 4 figures, plus 4 pages and 2 figures of supplemental material
نوع الوثيقة: Working Paper
DOI: 10.1063/5.0150891
URL الوصول: http://arxiv.org/abs/2305.19405
رقم الأكسشن: edsarx.2305.19405
قاعدة البيانات: arXiv