Imaging the Meissner effect and flux trapping in a hydride superconductor at megabar pressures using a nanoscale quantum sensor

التفاصيل البيبلوغرافية
العنوان: Imaging the Meissner effect and flux trapping in a hydride superconductor at megabar pressures using a nanoscale quantum sensor
المؤلفون: Bhattacharyya, Prabudhya, Chen, Wuhao, Huang, Xiaoli, Chatterjee, Shubhayu, Huang, Benchen, Kobrin, Bryce, Lyu, Yuanqi, Smart, Thomas J., Block, Maxwell, Wang, Esther, Wang, Zhipan, Wu, Weijie, Hsieh, Satcher, Ma, He, Mandyam, Srinivas, Chen, Bijuan, Davis, Emily, Geballe, Zachary M., Zu, Chong, Struzhkin, Viktor, Jeanloz, Raymond, Moore, Joel E., Cui, Tian, Galli, Giulia, Halperin, Bertrand I., Laumann, Chris R., Yao, Norman Y.
المصدر: Nature 627, 73-79 (2024)
سنة النشر: 2023
المجموعة: Condensed Matter
Quantum Physics
مصطلحات موضوعية: Condensed Matter - Superconductivity, Condensed Matter - Disordered Systems and Neural Networks, Quantum Physics
الوصف: By directly altering microscopic interactions, pressure provides a powerful tuning knob for the exploration of condensed phases and geophysical phenomena. The megabar regime represents an exciting frontier, where recent discoveries include novel high-temperature superconductors, as well as structural and valence phase transitions. However, at such high pressures, many conventional measurement techniques fail. Here, we demonstrate the ability to perform local magnetometry inside of a diamond anvil cell with sub-micron spatial resolution at megabar pressures. Our approach utilizes a shallow layer of Nitrogen-Vacancy (NV) color centers implanted directly within the anvil; crucially, we choose a crystal cut compatible with the intrinsic symmetries of the NV center to enable functionality at megabar pressures. We apply our technique to characterize a recently discovered hydride superconductor, CeH$_9$. By performing simultaneous magnetometry and electrical transport measurements, we observe the dual signatures of superconductivity: local diamagnetism characteristic of the Meissner effect and a sharp drop of the resistance to near zero. By locally mapping the Meissner effect and flux trapping, we directly image the geometry of superconducting regions, revealing significant inhomogeneities at the micron scale. Our work brings quantum sensing to the megabar frontier and enables the closed loop optimization of superhydride materials synthesis.
نوع الوثيقة: Working Paper
DOI: 10.1038/s41586-024-07026-7
URL الوصول: http://arxiv.org/abs/2306.03122
رقم الأكسشن: edsarx.2306.03122
قاعدة البيانات: arXiv
الوصف
DOI:10.1038/s41586-024-07026-7