Quantum Noise Spectroscopy of Criticality in an Atomically Thin Magnet

التفاصيل البيبلوغرافية
العنوان: Quantum Noise Spectroscopy of Criticality in an Atomically Thin Magnet
المؤلفون: Ziffer, Mark E., Machado, Francisco, Ursprung, Benedikt, Lozovoi, Artur, Tazi, Aya Batoul, Yuan, Zhiyang, Ziebel, Michael E., Delord, Tom, Zeng, Nanyu, Telford, Evan, Chica, Daniel G., deQuilettes, Dane W., Zhu, Xiaoyang, Hone, James C., Shepard, Kenneth L., Roy, Xavier, de Leon, Nathalie P., Davis, Emily J., Chatterjee, Shubhayu, Meriles, Carlos A., Owen, Jonathan S., Schuck, P. James, Pasupathy, Abhay N.
سنة النشر: 2024
المجموعة: Condensed Matter
Quantum Physics
مصطلحات موضوعية: Condensed Matter - Mesoscale and Nanoscale Physics, Quantum Physics
الوصف: Dynamic critical fluctuations in magnetic materials encode important information about magnetic ordering in the associated critical exponents. Using nitrogen-vacancy centers in diamond, we implement $T_2$ (spin-decoherence) noise magnetometry to study critical dynamics in a 2D Van der Waals magnet CrSBr. By analyzing NV decoherence on time scales approaching the characteristic correlation time $\tau_c$ of critical fluctuations, we extract the critical exponent $\nu$ for the correlation length. Our result deviates from the Ising prediction and highlights the role of long-range dipolar interactions in 2D CrSBr. Furthermore, analyzing the divergence of the correlation length suggests the possibility of 2D-XY criticality in CrSBr in a temperature window near $T_C$ where static magnetic domains are absent. Our work provides a first demonstration of $T_2$ noise magnetometry to quantitatively analyze critical scaling behavior in 2D materials.
Comment: 19 pages main text, 4 main text figures, 26 pages Supplementary Materials, 13 Supplementary figures
نوع الوثيقة: Working Paper
URL الوصول: http://arxiv.org/abs/2407.05614
رقم الأكسشن: edsarx.2407.05614
قاعدة البيانات: arXiv