دورية أكاديمية
أعرض في EDS

Tuning charge and correlation effects for a single molecule on a graphene device.

التفاصيل البيبلوغرافية
العنوان: Tuning charge and correlation effects for a single molecule on a graphene device.
المؤلفون: Wickenburg S; Department of Physics, University of California, Berkeley, California 94720, USA.; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA., Lu J; Department of Physics, University of California, Berkeley, California 94720, USA.; Department of Chemistry, National University of Singapore, 3 Science Drive 3, Singapore 117543, Singapore.; Centre for Advanced 2D Materials and Graphene Research National University of Singapore, 6 Science Drive 2, 117546 Singapore, Singapore., Lischner J; Department of Physics, University of California, Berkeley, California 94720, USA.; Department of Materials, Imperial College London, Prince Consort Rd, London SW7 2BB, UK., Tsai HZ; Department of Physics, University of California, Berkeley, California 94720, USA., Omrani AA; Department of Physics, University of California, Berkeley, California 94720, USA., Riss A; Department of Physics, University of California, Berkeley, California 94720, USA.; Physik-Department E20, Technical University of Munich, 85748 Garching, Germany., Karrasch C; Department of Physics, University of California, Berkeley, California 94720, USA.; Dahlem Center for Complex Quantum Systems and Fachbereich Physik, Freie Universität Berlin, 14195 Berlin, Germany., Bradley A; Department of Physics, University of California, Berkeley, California 94720, USA., Jung HS; Department of Physics, University of California, Berkeley, California 94720, USA., Khajeh R; Department of Physics, University of California, Berkeley, California 94720, USA., Wong D; Department of Physics, University of California, Berkeley, California 94720, USA., Watanabe K; National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan., Taniguchi T; National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044, Japan., Zettl A; Department of Physics, University of California, Berkeley, California 94720, USA.; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.; Kavli Energy NanoSciences Institute at the University of California Berkeley and the Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA., Neto AHC; Centre for Advanced 2D Materials and Graphene Research National University of Singapore, 6 Science Drive 2, 117546 Singapore, Singapore.; Department of Physics, National University of Singapore, 2 Science Drive 3, Singapore 117542, Singapore., Louie SG; Department of Physics, University of California, Berkeley, California 94720, USA.; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA., Crommie MF; Department of Physics, University of California, Berkeley, California 94720, USA.; Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.; Kavli Energy NanoSciences Institute at the University of California Berkeley and the Lawrence Berkeley National Laboratory, Berkeley, California 94720, USA.
المصدر: Nature communications [Nat Commun] 2016 Nov 25; Vol. 7, pp. 13553. Date of Electronic Publication: 2016 Nov 25.
نوع المنشور: Journal Article; Research Support, U.S. Gov't, Non-P.H.S.; Research Support, Non-U.S. Gov't
اللغة: English
بيانات الدورية: Publisher: Nature Pub. Group Country of Publication: England NLM ID: 101528555 Publication Model: Electronic Cited Medium: Internet ISSN: 2041-1723 (Electronic) Linking ISSN: 20411723 NLM ISO Abbreviation: Nat Commun Subsets: PubMed not MEDLINE
أسماء مطبوعة: Original Publication: [London] : Nature Pub. Group
مستخلص: The ability to understand and control the electronic properties of individual molecules in a device environment is crucial for developing future technologies at the nanometre scale and below. Achieving this, however, requires the creation of three-terminal devices that allow single molecules to be both gated and imaged at the atomic scale. We have accomplished this by integrating a graphene field effect transistor with a scanning tunnelling microscope, thus allowing gate-controlled charging and spectroscopic interrogation of individual tetrafluoro-tetracyanoquinodimethane molecules. We observe a non-rigid shift in the molecule's lowest unoccupied molecular orbital energy (relative to the Dirac point) as a function of gate voltage due to graphene polarization effects. Our results show that electron-electron interactions play an important role in how molecular energy levels align to the graphene Dirac point, and may significantly influence charge transport through individual molecules incorporated in graphene-based nanodevices.
References: Nat Chem. 2010 Oct;2(10):821-5. (PMID: 20861896)
Phys Rev Lett. 2004 Dec 3;93(23):236802. (PMID: 15601185)
ACS Nano. 2014 Jun 24;8(6):5395-401. (PMID: 24746016)
Nat Nanotechnol. 2013 Apr;8(4):282-7. (PMID: 23503093)
Nano Lett. 2011 Jun 8;11(6):2291-5. (PMID: 21553853)
Adv Mater. 2009 Nov 20;21(43):4303-22. (PMID: 26042937)
Phys Rev Lett. 2004 May 21;92(20):206102. (PMID: 15169370)
Nat Mater. 2006 Dec;5(12):995-1002. (PMID: 17128259)
Science. 2016 Jun 17;352(6292):1443-5. (PMID: 27313042)
Science. 2009 Jun 5;324(5932):1312-4. (PMID: 19423775)
Science. 2015 Apr 17;348(6232):308-11. (PMID: 25791086)
J Phys Condens Matter. 2009 Oct 7;21(40):402001. (PMID: 21832401)
Phys Rev Lett. 2014 Oct 31;113(18):186102. (PMID: 25396382)
Nature. 2009 Dec 24;462(7276):1039-43. (PMID: 20033044)
Science. 2009 Aug 28;325(5944):1110-4. (PMID: 19713523)
Phys Rev Lett. 2005 Oct 14;95(16):166103. (PMID: 16241819)
Science. 2001 Oct 19;294(5542):571-4. (PMID: 11641492)
Nat Nanotechnol. 2009 Sep;4(9):551-6. (PMID: 19734925)
Phys Rev Lett. 2013 Mar 29;110(13):136101. (PMID: 23581345)
Nat Nanotechnol. 2011 Jan;6(1):23-7. (PMID: 21076405)
Nature. 2002 Jun 13;417(6890):725-9. (PMID: 12066180)
Phys Rev Lett. 2012 Jan 20;108(3):036801. (PMID: 22400769)
Nature. 2003 Oct 16;425(6959):698-701. (PMID: 14562098)
Nature. 2000 Nov 30;408(6812):541-8. (PMID: 11117734)
Chem Soc Rev. 2015 Feb 21;44(4):902-19. (PMID: 25310767)
Science. 2012 Sep 14;337(6100):1326-9. (PMID: 22984067)
Nano Lett. 2013;13(12):5763-70. (PMID: 23464881)
Science. 2013 Nov 1;342(6158):611-4. (PMID: 24072819)
Science. 2004 Apr 9;304(5668):281-4. (PMID: 15016961)
Phys Rev Lett. 2006 Nov 24;97(21):216405. (PMID: 17155759)
Science. 2013 Jun 21;340(6139):1434-7. (PMID: 23722428)
Science. 2003 Aug 29;301(5637):1221-3. (PMID: 12947193)
Nature. 2000 Sep 7;407(6800):57-60. (PMID: 10993069)
Nanoscale. 2014 Dec 21;6(24):15271-9. (PMID: 25382549)
Nat Nanotechnol. 2013 Jun;8(6):399-410. (PMID: 23736215)
Phys Rev Lett. 2010 Jan 22;104(3):036805. (PMID: 20366671)
Rev Sci Instrum. 2007 Jan;78(1):013705. (PMID: 17503926)
Chem Soc Rev. 2014 Nov 7;43(21):7378-411. (PMID: 25099384)
Nat Nanotechnol. 2006 Dec;1(3):173-81. (PMID: 18654182)
Chem Commun (Camb). 2010 Nov 21;46(43):8198-200. (PMID: 20927433)
Science. 2010 Dec 24;330(6012):1807-10. (PMID: 21148345)
تواريخ الأحداث: Date Created: 20161126 Date Completed: 20180816 Latest Revision: 20190416
رمز التحديث: 20231215
مُعرف محوري في PubMed: PMC5133630
DOI: 10.1038/ncomms13553
PMID: 27886170
قاعدة البيانات: MEDLINE
الوصف
تدمد:2041-1723
DOI:10.1038/ncomms13553