دورية أكاديمية

Environmental and dietary exposure of perfluorooctanoic acid and perfluorooctanesulfonic acid in the Nakdong River, Korea.

التفاصيل البيبلوغرافية
العنوان: Environmental and dietary exposure of perfluorooctanoic acid and perfluorooctanesulfonic acid in the Nakdong River, Korea.
المؤلفون: Choi GH; Chemical Safety Division, National Institute of Agriculture Science, RDA, Wanju, 55365, Republic of Korea., Lee DY; Department of Agricultural Chemistry, Institute of Agriculture and Life Science (IALS), Gyeongsang National University, Jinju, 52828, Republic of Korea., Bruce-Vanderpuije P; Chemical Safety Division, National Institute of Agriculture Science, RDA, Wanju, 55365, Republic of Korea.; CSIR Water Research Institute, P. O. Box AH 38, Achimota, Accra, Ghana., Song AR; Chemical Safety Division, National Institute of Agriculture Science, RDA, Wanju, 55365, Republic of Korea., Lee HS; Chemical Safety Division, National Institute of Agriculture Science, RDA, Wanju, 55365, Republic of Korea., Park SW; Chemical Safety Division, National Institute of Agriculture Science, RDA, Wanju, 55365, Republic of Korea., Lee JH; Department of Life Resource Industry, Dong-A University, Busan, 49315, Republic of Korea., Megson D; Ecology and Environment Research Centre, Manchester Metropolitan University, Manchester, M1 5GD, UK., Kim JH; Department of Agricultural Chemistry, Institute of Agriculture and Life Science (IALS), Gyeongsang National University, Jinju, 52828, Republic of Korea. jhkim75@gnu.ac.kr.
المصدر: Environmental geochemistry and health [Environ Geochem Health] 2021 Jan; Vol. 43 (1), pp. 347-360. Date of Electronic Publication: 2020 Sep 18.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Kluwer Academic Publishers Country of Publication: Netherlands NLM ID: 8903118 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1573-2983 (Electronic) Linking ISSN: 02694042 NLM ISO Abbreviation: Environ Geochem Health Subsets: MEDLINE
أسماء مطبوعة: Publication: 1999- : Dordrecht : Kluwer Academic Publishers
Original Publication: Kew, Surrey : Science and Technology Letters, 1985-
مواضيع طبية MeSH: Alkanesulfonic Acids/*analysis , Caprylates/*analysis , Dietary Exposure/*analysis , Fluorocarbons/*analysis , Rivers/*chemistry , Water Pollutants, Chemical/*analysis, Animals ; Crops, Agricultural/metabolism ; Dietary Exposure/standards ; Food Contamination/analysis ; Humans ; Republic of Korea
مستخلص: This study performed the first environmental and dietary exposure assessment to explore plant uptake of perfluorooctanoic acid (PFOA) and perfluorooctanesulfonic acid (PFOS) from agricultural soil and irrigation water in the Nakdong River delta, South Korea. Annual average concentrations of total PFOA and PFOS ranged from 0.026 to 0.112 µg L -1 (irrigation water), and from 0.818 to 1.364 µg kg -1 (soil), respectively. PFOA and PFOS hotspots were identified downstream of the Nakdong River and were influenced by seasonal climatic variations. The observed average biennial concentration of the sum of PFOA and PFOS decreased in irrigation water, from 0.112 µg L -1 in 2013 to 0.026 µg L -1 in 2015, suggests that the 2013 Persistent Organic Pollutants Control Act may have helped to reduce levels of PFAS at this location. This study calculated some of the highest plant uptake factors reported to date, with values ranging from 0.962 in green onions to < 0.004 in plums. Leafy vegetables and rice are important components of the Korean diet; these groups had the largest contribution to the estimated dietary intake of PFOA and PFOS, which was calculated at 0.449 and 0.140 ng kg bw -1 day -1 , respectively. This corresponded to 66.4% for PFOA and 7.9% for PFOS of the EFSA reference dose (RfD). The dietary intake of PFOA and PFOS from crops alone did not exceed the RfD. However, when the estimated daily intake (EDI) from other sources such as tap water, meat, fish, dairy, and beverages was included in the exposure risk assessment, both of the EDIs to PFOA and PFOS exceeded the RfDs, indicating that there may be a risk to human health. This study concludes that consumption of crops might, therefore, be a significant and underappreciated pathway for human exposure to PFAS.
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معلومات مُعتمدة: PJ00930101 Rural Development Administration; PJ01332102 Rural Development Administration
فهرسة مساهمة: Keywords: Agricultural environment; Crop uptake; Estimated daily intakes; PFAS; PFOA; PFOS
المشرفين على المادة: 0 (Alkanesulfonic Acids)
0 (Caprylates)
0 (Fluorocarbons)
0 (Water Pollutants, Chemical)
947VD76D3L (perfluorooctanoic acid)
9H2MAI21CL (perfluorooctane sulfonic acid)
تواريخ الأحداث: Date Created: 20200919 Date Completed: 20210212 Latest Revision: 20210212
رمز التحديث: 20231215
DOI: 10.1007/s10653-020-00721-0
PMID: 32949006
قاعدة البيانات: MEDLINE
الوصف
تدمد:1573-2983
DOI:10.1007/s10653-020-00721-0