دورية أكاديمية
Performing calculus: Asymmetric adaptive stimuli-responsive material for derivative control.
العنوان: | Performing calculus: Asymmetric adaptive stimuli-responsive material for derivative control. |
---|---|
المؤلفون: | Gonuguntla S; Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, Singapore 117585, Singapore., Lim WC; Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, Singapore 117585, Singapore., Leong FY; A*STAR Institute of High Performance Computing, 1 Fusionopolis Way, Connexis, Singapore 138632, Singapore., Ao CK; Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, Singapore 117585, Singapore., Liu C; Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, Singapore 117585, Singapore., Soh S; Department of Chemical and Biomolecular Engineering, National University of Singapore, 4 Engineering Drive 4, Singapore 117585, Singapore. chessl@nus.edu.sg. |
المصدر: | Science advances [Sci Adv] 2021 Mar 31; Vol. 7 (14). Date of Electronic Publication: 2021 Mar 31 (Print Publication: 2021). |
نوع المنشور: | Journal Article |
اللغة: | English |
بيانات الدورية: | Publisher: American Association for the Advancement of Science Country of Publication: United States NLM ID: 101653440 Publication Model: Electronic-Print Cited Medium: Internet ISSN: 2375-2548 (Electronic) Linking ISSN: 23752548 NLM ISO Abbreviation: Sci Adv Subsets: PubMed not MEDLINE; MEDLINE |
أسماء مطبوعة: | Original Publication: Washington, DC : American Association for the Advancement of Science, [2015]- |
مستخلص: | Materials (e.g., brick or wood) are generally perceived as unintelligent. Even the highly researched "smart" materials are only capable of extremely primitive analytical functions (e.g., simple logical operations). Here, a material is shown to have the ability to perform (i.e., without a computer), an advanced mathematical operation in calculus: the temporal derivative. It consists of a stimuli-responsive material coated asymmetrically with an adaptive impermeable layer. Its ability to analyze the derivative is shown by experiments, numerical modeling, and theory (i.e., scaling between derivative and response). This class of freestanding stimuli-responsive materials is demonstrated to serve effectively as a derivative controller for controlled delivery and self-regulation. Its fast response realizes the same designed functionality and efficiency as complex industrial derivative controllers widely used in manufacturing. These results illustrate the possibility to associate specifically designed materials directly with higher concepts of mathematics for the development of "intelligent" material-based systems. (Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC).) |
References: | Adv Mater. 2020 Apr;32(13):e1902004. (PMID: 31423670) Chem Soc Rev. 2018 Apr 3;47(7):2228-2248. (PMID: 29493684) Adv Mater. 2015 Jul 15;27(27):4062-8. (PMID: 26043083) Adv Mater. 2015 Dec 16;27(47):7847-53. (PMID: 26498272) Sci Rep. 2017 Mar 10;7:44208. (PMID: 28281646) Adv Drug Deliv Rev. 2006 Dec 30;58(15):1655-70. (PMID: 17125884) Int J Pharm. 2006 Aug 17;319(1-2):29-36. (PMID: 16677786) Science. 1995 Jul 28;269(5223):525-7. (PMID: 17842364) J Am Chem Soc. 2018 Apr 25;140(16):5356-5359. (PMID: 29617118) Chem Rev. 2008 Jul;108(7):2482-505. (PMID: 18465900) J Am Chem Soc. 2009 Aug 19;131(32):11344-6. (PMID: 19624127) Nat Mater. 2010 Feb;9(2):101-13. (PMID: 20094081) J Control Release. 2001 Jun 15;73(2-3):121-36. (PMID: 11516493) Angew Chem Int Ed Engl. 2012 Feb 6;51(6):1420-3. (PMID: 22105942) Chem Soc Rev. 2013 Sep 7;42(17):7148-60. (PMID: 23749141) Nature. 2011 Jul 20;475(7356):368-72. (PMID: 21776082) ACS Nano. 2018 Jun 26;12(6):5452-5462. (PMID: 29750502) Chem Soc Rev. 2013 Sep 7;42(17):7055-6. (PMID: 23881304) Nature. 2012 Jul 11;487(7406):214-8. (PMID: 22785318) Nature. 2000 Apr 6;404(6778):588-90. (PMID: 10766238) ACS Nano. 2018 Mar 27;12(3):2466-2473. (PMID: 29455516) Adv Mater. 2017 May;29(18):. (PMID: 28247973) Adv Mater. 2019 Mar;31(11):e1804540. (PMID: 30624820) New Phytol. 2017 Mar;213(4):1818-1835. (PMID: 27933609) Chem Soc Rev. 2012 Sep 21;41(18):6042-65. (PMID: 22618080) Ann Bot. 2017 Jun 1;119(8):1365-1383. (PMID: 28334385) Chem Commun (Camb). 2018 Sep 25;54(77):10909-10912. (PMID: 30206617) Int J Pharm. 2018 Dec 1;552(1-2):301-311. (PMID: 30291961) Adv Mater. 2018 Jun;30(26):e1800109. (PMID: 29761554) Polymers (Basel). 2020 Sep 18;12(9):. (PMID: 32962059) Nat Mater. 2015 Aug;14(8):790-5. (PMID: 26099112) J Am Chem Soc. 2004 Mar 17;126(10):3032-3. (PMID: 15012116) Science. 2007 Feb 23;315(5815):1116-20. (PMID: 17322058) Nat Commun. 2016 Jun 27;7:12028. (PMID: 27345380) Angew Chem Int Ed Engl. 2017 Oct 2;56(41):12581-12585. (PMID: 28772021) Angew Chem Int Ed Engl. 2012 Feb 27;51(9):2124-8. (PMID: 22162189) J Am Chem Soc. 2009 Apr 22;131(15):5580-5. (PMID: 19331364) Chem Commun (Camb). 2011 Jan 14;47(2):665-7. (PMID: 21113530) Angew Chem Int Ed Engl. 2011 Apr 26;50(18):4103-7. (PMID: 21452185) |
تواريخ الأحداث: | Date Created: 20210401 Latest Revision: 20240501 |
رمز التحديث: | 20240501 |
مُعرف محوري في PubMed: | PMC8011968 |
DOI: | 10.1126/sciadv.abe5698 |
PMID: | 33789896 |
قاعدة البيانات: | MEDLINE |
تدمد: | 2375-2548 |
---|---|
DOI: | 10.1126/sciadv.abe5698 |