دورية أكاديمية
أعرض في EDS

Development of Fluorine-Free Tantalum Carbide MXene Hybrid Structure as a Biocompatible Material for Supercapacitor Electrodes.

التفاصيل البيبلوغرافية
العنوان: Development of Fluorine-Free Tantalum Carbide MXene Hybrid Structure as a Biocompatible Material for Supercapacitor Electrodes.
المؤلفون: Rafieerad A; Regenerative Medicine Program Institute of Cardiovascular Sciences St. Boniface Hospital Research Centre Department of Physiology and Pathophysiology Rady Faculty of Health Sciences University of Manitoba Winnipeg MB R2H 0G1 Canada., Amiri A; J. Mike Walker '66 Mechanical Engineering Department Texas A&M University College Station TX 77843 USA., Sequiera GL; Regenerative Medicine Program Institute of Cardiovascular Sciences St. Boniface Hospital Research Centre Department of Physiology and Pathophysiology Rady Faculty of Health Sciences University of Manitoba Winnipeg MB R2H 0G1 Canada., Yan W; Regenerative Medicine Program Institute of Cardiovascular Sciences St. Boniface Hospital Research Centre Department of Physiology and Pathophysiology Rady Faculty of Health Sciences University of Manitoba Winnipeg MB R2H 0G1 Canada., Chen Y; Department of Aerospace Engineering Texas A&M University College Station TX 77843 USA., Polycarpou AA; J. Mike Walker '66 Mechanical Engineering Department Texas A&M University College Station TX 77843 USA., Dhingra S; Regenerative Medicine Program Institute of Cardiovascular Sciences St. Boniface Hospital Research Centre Department of Physiology and Pathophysiology Rady Faculty of Health Sciences University of Manitoba Winnipeg MB R2H 0G1 Canada.
المصدر: Advanced functional materials [Adv Funct Mater] 2021 Jul 23; Vol. 31 (30), pp. 2100015. Date of Electronic Publication: 2021 May 24.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 101190390 Publication Model: Print-Electronic Cited Medium: Print ISSN: 1616-301X (Print) Linking ISSN: 1616301X NLM ISO Abbreviation: Adv Funct Mater Subsets: PubMed not MEDLINE
أسماء مطبوعة: Original Publication: Weinheim, Germany : Wiley-VCH, c2001-
مستخلص: The application of nontoxic 2D transition-metal carbides (MXenes) has recently gained ground in bioelectronics. In group-4 transition metals, tantalum possesses enhanced biological and physical properties compared to other MXene counterparts. However, the application of tantalum carbide for bioelectrodes has not yet been explored. Here, fluorine-free exfoliation and functionalization of tantalum carbide MAX-phase to synthesize a novel Ta 4 C 3 T x MXene-tantalum oxide (TTO) hybrid structure through an innovative, facile, and inexpensive protocol is demonstrated. Additionally, the application of TTO composite as an efficient biocompatible material for supercapacitor electrodes is reported. The TTO electrode displays long-term stability over 10 000 cycles with capacitance retention of over 90% and volumetric capacitance of 447 F cm -3  (194 F g -1 ) at 1 mV s -1 . Furthermore, TTO shows excellent biocompatibility with human-induced pluripotent stem cells-derived cardiomyocytes, neural progenitor cells, fibroblasts, and mesenchymal stem cells. More importantly, the electrochemical data show that TTO outperforms most of the previously reported biomaterials-based supercapacitors in terms of gravimetric/volumetric energy and power densities. Therefore, TTO hybrid structure may open a gateway as a bioelectrode material with high energy-storage performance for size-sensitive applications.
Competing Interests: The authors declare no conflict of interest.
(© 2021 The Authors. Advanced Functional Materials published by Wiley‐VCH GmbH.)
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فهرسة مساهمة: Keywords: Ta 4C 3Tx MXene‐tantalum oxide; biocompatible electrode; fluorine‐free Ta 4C 3Tx MXene; human stem cells; hybrid structures; supercapacitors
تواريخ الأحداث: Date Created: 20220310 Latest Revision: 20220311
رمز التحديث: 20221213
مُعرف محوري في PubMed: PMC8889894
DOI: 10.1002/adfm.202100015
PMID: 35264918
قاعدة البيانات: MEDLINE
الوصف
تدمد:1616-301X
DOI:10.1002/adfm.202100015