دورية أكاديمية

Visualizing Atomically Layered Magnetism in CrSBr.

التفاصيل البيبلوغرافية
العنوان: Visualizing Atomically Layered Magnetism in CrSBr.
المؤلفون: Rizzo DJ; Department of Physics, Columbia University, New York, NY, 10027, USA., McLeod AS; Department of Physics, Columbia University, New York, NY, 10027, USA., Carnahan C; Department of Physics, Carnegie Mellon University, Pittsburgh, PA, 15213, USA., Telford EJ; Department of Physics, Columbia University, New York, NY, 10027, USA.; Department of Chemistry, Columbia University, New York, NY, 10027, USA., Dismukes AH; Department of Chemistry, Columbia University, New York, NY, 10027, USA., Wiscons RA; Department of Chemistry, Columbia University, New York, NY, 10027, USA., Dong Y; Department of Physics, Columbia University, New York, NY, 10027, USA., Nuckolls C; Department of Chemistry, Columbia University, New York, NY, 10027, USA., Dean CR; Department of Physics, Columbia University, New York, NY, 10027, USA., Pasupathy AN; Department of Physics, Columbia University, New York, NY, 10027, USA., Roy X; Department of Chemistry, Columbia University, New York, NY, 10027, USA., Xiao D; Department of Material Science and Engineering, University of Washington, Seattle, WA, 98195, USA.; Department of Physics, University of Washington, Seattle, WA, 98195, USA., Basov DN; Department of Physics, Columbia University, New York, NY, 10027, USA.
المصدر: Advanced materials (Deerfield Beach, Fla.) [Adv Mater] 2022 Jul; Vol. 34 (27), pp. e2201000. Date of Electronic Publication: 2022 May 31.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 9885358 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-4095 (Electronic) Linking ISSN: 09359648 NLM ISO Abbreviation: Adv Mater Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Publication: Sept. 3, 1997- : Weinheim : Wiley-VCH
Original Publication: Deerfield Beach, FL : VCH Publishers, 1989-
مستخلص: 2D materials can host long-range magnetic order in the presence of underlying magnetic anisotropy. The ability to realize the full potential of 2D magnets necessitates systematic investigation of the role of individual atomic layers and nanoscale inhomogeneity (i.e., strain) on the emergence of stable magnetic phases. Here, spatially dependent magnetism in few-layer CrSBr is revealed using magnetic force microscopy (MFM) and Monte Carlo-based simulations. Nanoscale visualization of the magnetic sheet susceptibility is extracted from MFM data and force-distance curves, revealing a characteristic onset of both intra- and interlayer magnetic correlations as a function of temperature and layer-thickness. These results demonstrate that the presence of a single uncompensated layer in odd-layer terraces significantly reduces the stability of the low-temperature antiferromagnetic (AFM) phase and gives rise to multiple coexisting magnetic ground states at temperatures close to the bulk Néel temperature (T N ). Furthermore, the AFM phase can be reliably suppressed using modest fields (≈16 mT) from the MFM probe, behaving as a nanoscale magnetic switch. This prototypical study of few-layer CrSBr demonstrates the critical role of layer parity on field-tunable 2D magnetism and validates MFM for use in nanomagnetometry of 2D materials (despite the ubiquitous absence of bulk zero-field magnetism in magnetized sheets).
(© 2022 Wiley-VCH GmbH.)
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معلومات مُعتمدة: DE-SC0019443 U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES); Arnold O. Beckman Fellowship in Chemical Sciences; DGE 16-44869 National Science Foundation graduate research fellowship programme
فهرسة مساهمة: Keywords: 2D magnets; 2D materials; magnetic force microscopy; magnetometry; van der Waals materials
تواريخ الأحداث: Date Created: 20220503 Latest Revision: 20220707
رمز التحديث: 20221213
DOI: 10.1002/adma.202201000
PMID: 35504841
قاعدة البيانات: MEDLINE
الوصف
تدمد:1521-4095
DOI:10.1002/adma.202201000