دورية أكاديمية

Application of response surface methodology and box-behnken design for the optimization of mercury removal by Ulva sp.

التفاصيل البيبلوغرافية
العنوان: Application of response surface methodology and box-behnken design for the optimization of mercury removal by Ulva sp.
المؤلفون: Ferreira N; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal., Viana T; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal., Henriques B; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal; Central Laboratory of Analysis, University of Aveiro, 3810-193 Aveiro, Portugal. Electronic address: brunogalinho@ua.pt., Tavares DS; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal., Jacinto J; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal., Colónia J; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal., Pinto J; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal., Pereira E; LAQV-REQUIMTE - Associated Laboratory for Green Chemistry, Department of Chemistry, University of Aveiro, 3810-193 Aveiro, Portugal; Central Laboratory of Analysis, University of Aveiro, 3810-193 Aveiro, Portugal.
المصدر: Journal of hazardous materials [J Hazard Mater] 2023 Mar 05; Vol. 445, pp. 130405. Date of Electronic Publication: 2022 Nov 17.
نوع المنشور: Journal Article; Research Support, Non-U.S. Gov't
اللغة: English
بيانات الدورية: Publisher: Elsevier Country of Publication: Netherlands NLM ID: 9422688 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1873-3336 (Electronic) Linking ISSN: 03043894 NLM ISO Abbreviation: J Hazard Mater Subsets: MEDLINE
أسماء مطبوعة: Original Publication: Amsterdam : Elsevier,
مواضيع طبية MeSH: Mercury* , Ulva* , Water Pollutants, Chemical*/analysis , Metals, Rare Earth* , Seaweed*, Salinity
مستخلص: Mercury (Hg) is a global and top priority contaminant, toxic at low concentrations. Although it has been progressively eliminated from processes, this metal continues to circulate in the atmosphere, soil, and water. In this work, the Response Surface Methodology (RSM) combined with a Box-Behnken Design (3 factors - 3 levels) was used to optimize key operational conditions that influence the removal and uptake of Hg by living macroalga Ulva sp. in a complex mixture containing several elements used in industry (potentially toxic elements, rare earth elements, and platinum-group elements) (initial concentration 10, 100 and 190 µg/L, salinity 15, 25 and 35, seaweed stock density 1.0, 3.0 and 5.0 g/L). Results evidenced the great capability of Ulva sp. to remove Hg, with removal efficiencies between 69 % and 97 %. 3-D surfaces showed that the most impactful variable was seaweed stock density, with higher densities leading to higher removal. Regarding the uptake, a positive correlation between initial concentration and q t values was observed. The appliance of RSM made possible to obtain optimal operating conditions for removing virtually 100 % of Hg from waters with high ionic strength, which is a pivotal step in the direction of the application of this remediation biotechnology at large scale.
Competing Interests: Declaration of Competing Interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.
(Copyright © 2022 The Authors. Published by Elsevier B.V. All rights reserved.)
فهرسة مساهمة: Keywords: Lamp industry; Macroalgae biotechnology; Mercury removal; Process optimization
المشرفين على المادة: FXS1BY2PGL (Mercury)
0 (Water Pollutants, Chemical)
0 (Metals, Rare Earth)
تواريخ الأحداث: Date Created: 20221127 Date Completed: 20230116 Latest Revision: 20230117
رمز التحديث: 20240829
DOI: 10.1016/j.jhazmat.2022.130405
PMID: 36437192
قاعدة البيانات: MEDLINE
الوصف
تدمد:1873-3336
DOI:10.1016/j.jhazmat.2022.130405