دورية أكاديمية
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Pore Aperture Control Toward Size-Exclusion-Based Hydrocarbon Separations.

التفاصيل البيبلوغرافية
العنوان: Pore Aperture Control Toward Size-Exclusion-Based Hydrocarbon Separations.
المؤلفون: Lal B; Department of Chemistry, Northwestern University, 60208, Evanston, IL, USA.; Institute of Chemistry, Shah Abdul Latif University, 66020, Khairpur, Sindh, Pakistan., Idrees KB; Department of Chemistry, Northwestern University, 60208, Evanston, IL, USA., Xie H; Department of Chemistry, Northwestern University, 60208, Evanston, IL, USA., Smoljan CS; Department of Chemical and Biological Engineering, Northwestern University, 60208, Evanston, IL, USA., Shafaie S; Integrated Molecular Structure and Education Center, Northwestern University, 60208, Evanston, IL, USA., Islamoglu T; Department of Chemistry, Northwestern University, 60208, Evanston, IL, USA., Farha OK; Department of Chemistry, Northwestern University, 60208, Evanston, IL, USA.; Department of Chemical and Biological Engineering, Northwestern University, 60208, Evanston, IL, USA.
المصدر: Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2023 Apr 11; Vol. 62 (16), pp. e202219053. Date of Electronic Publication: 2023 Mar 06.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 0370543 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-3773 (Electronic) Linking ISSN: 14337851 NLM ISO Abbreviation: Angew Chem Int Ed Engl Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Publication: <2004-> : Weinheim : Wiley-VCH
Original Publication: Weinheim/Bergstr. : New York, : Verlag Chemie ; Academic Press, c1962-
مستخلص: Metal-organic frameworks (MOFs) have been proposed as a promising material for non-thermal chemical separations owing to their high structural diversity and tunability. Here, we report the synthesis of a zinc-based MOF containing a three-dimensional (3D) linker, bicyclo[2.2.2]octane-1,4-dicarboxylic acid, with high thermal stability towards the separation of hexane isomers. The incorporation of the 3D linker enhances the structural stability and provides well-defined pore apertures/channels with sub-Ångstrom precision. This precision allowed for the separation of similarly sized hexane isomers based on subtle differences in their kinetic diameters. Multi-component liquid phase batch experiments confirmed the separation of hexanes mixture into linear, monobranched, and dibranched isomers. This work represents a significant milestone in the construction of stable Zn-based MOFs and the incorporation of 3D linkers as a potential solution to challenging separations.
(© 2023 Wiley-VCH GmbH.)
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معلومات مُعتمدة: DE-FG02-08ER15967 Office of Science
فهرسة مساهمة: Keywords: Hexanes; Metal-Organic Frameworks; Separation; Zn-MOF
تواريخ الأحداث: Date Created: 20230215 Date Completed: 20230403 Latest Revision: 20230403
رمز التحديث: 20240628
DOI: 10.1002/anie.202219053
PMID: 36790793
قاعدة البيانات: MEDLINE
الوصف
تدمد:1521-3773
DOI:10.1002/anie.202219053