دورية أكاديمية
Zirconium preconcentration from zircon raffinate using gamma radiation-induced polymerization of reduced graphene oxide composite.
| العنوان: | Zirconium preconcentration from zircon raffinate using gamma radiation-induced polymerization of reduced graphene oxide composite. |
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| المؤلفون: | Ali AH; Nuclear Materials Authority, Maadi, P.O. 530, Cairo, Egypt., Abdo SM; Nuclear Materials Authority, Maadi, P.O. 530, Cairo, Egypt., Dakroury GARS; Nuclear Chemistry Department, Hot Laboratories Centre, Egyptian Atomic Energy Authority, P.O. 13759, Cairo, Egypt. dr_gdakrory2010@yahoo.com. |
| المصدر: | Environmental science and pollution research international [Environ Sci Pollut Res Int] 2023 Apr; Vol. 30 (20), pp. 58330-58345. Date of Electronic Publication: 2023 Mar 29. |
| نوع المنشور: | Journal Article |
| اللغة: | English |
| بيانات الدورية: | Publisher: Springer Country of Publication: Germany NLM ID: 9441769 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1614-7499 (Electronic) Linking ISSN: 09441344 NLM ISO Abbreviation: Environ Sci Pollut Res Int Subsets: MEDLINE |
| أسماء مطبوعة: | Publication: <2013->: Berlin : Springer Original Publication: Landsberg, Germany : Ecomed |
| مواضيع طبية MeSH: | Zirconium*/chemistry, Gamma Rays ; Polymerization ; Adsorption ; Hydrogen-Ion Concentration ; Kinetics |
| مستخلص: | Zirconium is commonly used as a cladding material for nuclear reactors. The purity of the zirconium material seeks to control reactor efficiency. A novel composite of reduced graphene oxide-grafted polyacrylic acid, malic acid, and trioctylamine (rGO-g-PAA-MA/TOA) was prepared using in situ radical polymerization with gamma radiation at a dose of 25 KGy from a 60 Co cell to preconcentrate zirconium Zr(IV) from zircon raffinate. Five distinct rGO-g-PAA-MA/TOA composite compositions were created and evaluated. The best composite composition was 62.95% acrylic acid, 15.8% malic acid, and 15.8% trioctylamine. After 60 min, the sorption reaction reached equilibrium at pH 0.35 and 20 °C. The pseudo n th order indicated that the order of the sorption reaction was 1.8476. The Elovich model and Dubinin-Radushkevich model controlled the kinetic mechanism and adsorption isotherm of the sorption reaction, respectively; based on estimated regression plots and quantitatively with three different error functions: coefficient of determination (R 2 ), chi-square statistic (χ 2 ), and corrected Akaike information (AIC (© 2023. The Author(s).) |
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| فهرسة مساهمة: | Keywords: Polyacrylic acid composite; Reduced graphene oxide; Sorption; Zircon raffinate zirconium preconcentration |
| المشرفين على المادة: | 0 (graphene oxide) I40965UY86 (tri-N-octylamine) 817L1N4CKP (malic acid) 4SY8H89134 (zircon) C6V6S92N3C (Zirconium) |
| تواريخ الأحداث: | Date Created: 20230328 Date Completed: 20230510 Latest Revision: 20230510 |
| رمز التحديث: | 20230512 |
| مُعرف محوري في PubMed: | PMC10163083 |
| DOI: | 10.1007/s11356-023-26485-5 |
| PMID: | 36977885 |
| قاعدة البيانات: | MEDLINE |
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Full Text Finder | تدمد: | 1614-7499 |
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| DOI: | 10.1007/s11356-023-26485-5 |