دورية أكاديمية
Electrochemical Doping of Halide Perovskites by Noble Metal Interstitial Cations.
العنوان: | Electrochemical Doping of Halide Perovskites by Noble Metal Interstitial Cations. |
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المؤلفون: | Kerner RA; National Renewable Energy Laboratory, Golden, CO, 80401, USA., Cohen AV; Department of Molecular Chemistry and Materials Science, Weizmann Institute of Science, Rehovoth, 76100, Israel., Xu Z; Department of Electrical Engineering, Princeton University, Princeton, NJ, 08544, USA., Kirmani AR; National Renewable Energy Laboratory, Golden, CO, 80401, USA., Park SY; National Renewable Energy Laboratory, Golden, CO, 80401, USA., Harvey SP; National Renewable Energy Laboratory, Golden, CO, 80401, USA., Murphy JP; Department of Electrical Engineering, The Pennsylvania State University, University Park, PA, 16802, USA., Cawthorn RC; Department of Electrical Engineering, The Pennsylvania State University, University Park, PA, 16802, USA., Giebink NC; Department of Electrical Engineering, The Pennsylvania State University, University Park, PA, 16802, USA., Luther JM; National Renewable Energy Laboratory, Golden, CO, 80401, USA., Zhu K; National Renewable Energy Laboratory, Golden, CO, 80401, USA., Berry JJ; National Renewable Energy Laboratory, Golden, CO, 80401, USA.; Department of Physics, University of Colorado Boulder, Boulder, CO, 80309, USA.; Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder, CO, 80309, USA., Kronik L; Department of Molecular Chemistry and Materials Science, Weizmann Institute of Science, Rehovoth, 76100, Israel., Rand BP; Department of Electrical Engineering, Princeton University, Princeton, NJ, 08544, USA.; Andlinger Center for Energy and the Environment, Princeton University, Princeton, NJ, 08544, USA. |
المصدر: | Advanced materials (Deerfield Beach, Fla.) [Adv Mater] 2023 Jul; Vol. 35 (29), pp. e2302206. Date of Electronic Publication: 2023 Jun 02. |
نوع المنشور: | Journal Article |
اللغة: | English |
بيانات الدورية: | Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 9885358 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-4095 (Electronic) Linking ISSN: 09359648 NLM ISO Abbreviation: Adv Mater Subsets: PubMed not MEDLINE; MEDLINE |
أسماء مطبوعة: | Publication: Sept. 3, 1997- : Weinheim : Wiley-VCH Original Publication: Deerfield Beach, FL : VCH Publishers, 1989- |
مستخلص: | Metal halide perovskites are an attractive class of semiconductors, but it has proven difficult to control their electronic doping by conventional strategies due to screening and compensation by mobile ions or ionic defects. Noble-metal interstitials represent an under-studied class of extrinsic defects that plausibly influence many perovskite-based devices. In this work, doping of metal halide perovskites is studied by electrochemically formed Au + interstitial ions, combining experimental data on devices with a computational analysis of Au + interstitial defects based on density functional theory (DFT). Analysis suggests that Au + cations can be easily formed and migrate through the perovskite bulk via the same sites as iodine interstitials (I (© 2023 The Authors. Advanced Materials published by Wiley-VCH GmbH.) |
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معلومات مُعتمدة: | DE-AC36-08GO28308 U.S. Department of Energy; DE-FOA-0000990 Advanced Perovskite Cells and Modules; NN66001-20-1-4052 Defense Advanced Research Projects Agency; N00014-21-1-2767 Office of Naval Research; CHOISE Energy Frontier Research Centers |
فهرسة مساهمة: | Keywords: electrochemical doping; halide perovskite; interstitial defects |
تواريخ الأحداث: | Date Created: 20230413 Latest Revision: 20230720 |
رمز التحديث: | 20240628 |
DOI: | 10.1002/adma.202302206 |
PMID: | 37052234 |
قاعدة البيانات: | MEDLINE |
تدمد: | 1521-4095 |
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DOI: | 10.1002/adma.202302206 |