دورية أكاديمية
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First report of trans -A 2 B-corrole derived from a lapachone derivative: photophysical, TD-DFT and photobiological assays.

التفاصيل البيبلوغرافية
العنوان: First report of trans -A 2 B-corrole derived from a lapachone derivative: photophysical, TD-DFT and photobiological assays.
المؤلفون: Rodrigues BM; Bioinorganic and Porphyrinoid Material Laboratory, Department of Chemistry, Federal University of Santa Maria Santa Maria-RS Brazil bernardo.iglesias@ufsm.br., Diniz CC; Bioinorganic and Porphyrinoid Material Laboratory, Department of Chemistry, Federal University of Santa Maria Santa Maria-RS Brazil bernardo.iglesias@ufsm.br., da Rocha VN; Department of Physics, Federal University of Santa Maria Santa Maria-RS Brazil., Köhler MH; Department of Physics, Federal University of Santa Maria Santa Maria-RS Brazil., Brandão GP; Department of Chemistry, Federal University of Minas Gerais Belo Horizonte MG Brazil., Machado LA; Department of Chemistry, Federal University of Minas Gerais Belo Horizonte MG Brazil.; Julius Maximilians-Universität Würzburg (JMU), Institute for Inorganic Chemistry Am Hubland Würzburg 97074 Germany., da Silva Júnior EN; Department of Chemistry, Federal University of Minas Gerais Belo Horizonte MG Brazil., Iglesias BA; Bioinorganic and Porphyrinoid Material Laboratory, Department of Chemistry, Federal University of Santa Maria Santa Maria-RS Brazil bernardo.iglesias@ufsm.br.
المصدر: RSC advances [RSC Adv] 2023 Apr 11; Vol. 13 (16), pp. 11121-11129. Date of Electronic Publication: 2023 Apr 11 (Print Publication: 2023).
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Royal Society of Chemistry Country of Publication: England NLM ID: 101581657 Publication Model: eCollection Cited Medium: Internet ISSN: 2046-2069 (Electronic) Linking ISSN: 20462069 NLM ISO Abbreviation: RSC Adv Subsets: PubMed not MEDLINE
أسماء مطبوعة: Original Publication: Cambridge [England] : Royal Society of Chemistry, [2011]-
مستخلص: In this work, the synthesis, characterization and photophysical assays of a new trans -A 2 B-corrole derivative from the naturally occurring quinone are described. β-Lapachone is a naturally occurring quinoidal compound that provides highly fluorescent heterocyclic compounds such as lapimidazoles. The new trans -A 2 B-corrole compound was obtained from the reaction between 2,3,4,5,6-(pentafluorophenyl)dipyrromethane and the lapimidazole bearing an aldehyde group. The dyad was characterized by high-resolution mass spectrometry (HRMS), NMR spectroscopy ( 1 H, COSY 2D, HMBC, 19 F), FT-IR, UV-vis, steady-state and time-resolved fluorescence, electrochemical studies (CV), TD-DFT analysis and photobiological experiments, in which includes aggregation, stability in solution, photostability and partition coefficients assays. Finally, ROS generation assays were performed using 1,3-diphenylisobenzofuran (DPBF) method and the presented compound showed significant photostability and singlet oxygen production.
Competing Interests: The authors declare that they do not have conflict of interest.
(This journal is © The Royal Society of Chemistry.)
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تواريخ الأحداث: Date Created: 20230414 Latest Revision: 20230415
رمز التحديث: 20230415
مُعرف محوري في PubMed: PMC10089255
DOI: 10.1039/d3ra00823a
PMID: 37056965
قاعدة البيانات: MEDLINE
الوصف
تدمد:2046-2069
DOI:10.1039/d3ra00823a