دورية أكاديمية
Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution.
| العنوان: | Design Rules for Obtaining Narrow Luminescence from Semiconductors Made in Solution. |
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| المؤلفون: | Nguyen HA; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Dixon G; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Dou FY; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Gallagher S; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Gibbs S; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Ladd DM; Department of Materials Science and Engineering, University of Colorado Boulder, Boulder, Colorado 80303, United States., Marino E; Department of Chemistry, University of Pennsylvania, Philadelphia, Pennsylvania 19104, United States.; Dipartimento di Fisica e Chimica, Università degli Studi di Palermo, Via Archirafi 36, 90123 Palermo, Italy., Ondry JC; Department of Chemistry, James Franck Institute, and Pritzker School of Molecular Engineering, University of Chicago, Chicago, Illinois 60637, United States., Shanahan JP; Department of Chemistry, Columbia University, New York, New York 10027, United States., Vasileiadou ES; Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States., Barlow S; Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder, Colorado 80303, United States., Gamelin DR; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Ginger DS; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States., Jonas DM; Department of Chemistry, University of Colorado Boulder, Boulder, Colorado 80309, United States.; Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder, Colorado 80303, United States., Kanatzidis MG; Department of Chemistry, Northwestern University, Evanston, Illinois 60208, United States., Marder SR; Department of Chemistry, University of Colorado Boulder, Boulder, Colorado 80309, United States.; Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder, Colorado 80303, United States.; Department of Chemical and Biological Engineering, University of Colorado Boulder, Boulder, Colorado 80303, United States., Morton D; Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder, Colorado 80303, United States., Murray CB; Department of Chemistry, University of Pennsylvania, Philadelphia, Pennsylvania 19104, United States., Owen JS; Department of Chemistry, Columbia University, New York, New York 10027, United States., Talapin DV; Department of Chemistry, James Franck Institute, and Pritzker School of Molecular Engineering, University of Chicago, Chicago, Illinois 60637, United States., Toney MF; Department of Materials Science and Engineering, University of Colorado Boulder, Boulder, Colorado 80303, United States.; Renewable and Sustainable Energy Institute, University of Colorado Boulder, Boulder, Colorado 80303, United States.; Department of Chemical and Biological Engineering, University of Colorado Boulder, Boulder, Colorado 80303, United States., Cossairt BM; Department of Chemistry, University of Washington, Seattle, Washington 98195-1700, United States. |
| المصدر: | Chemical reviews [Chem Rev] 2023 Jun 28; Vol. 123 (12), pp. 7890-7952. Date of Electronic Publication: 2023 Jun 13. |
| نوع المنشور: | Journal Article; Review |
| اللغة: | English |
| بيانات الدورية: | Publisher: American Chemical Society Country of Publication: United States NLM ID: 2985134R Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1520-6890 (Electronic) Linking ISSN: 00092665 NLM ISO Abbreviation: Chem Rev Subsets: PubMed not MEDLINE; MEDLINE |
| أسماء مطبوعة: | Publication: Washington, DC : American Chemical Society Original Publication: Easton, Pa. [etc.] American Chemical Society. |
| مستخلص: | Solution-processed semiconductors are in demand for present and next-generation optoelectronic technologies ranging from displays to quantum light sources because of their scalability and ease of integration into devices with diverse form factors. One of the central requirements for semiconductors used in these applications is a narrow photoluminescence (PL) line width. Narrow emission line widths are needed to ensure both color and single-photon purity, raising the question of what design rules are needed to obtain narrow emission from semiconductors made in solution. In this review, we first examine the requirements for colloidal emitters for a variety of applications including light-emitting diodes, photodetectors, lasers, and quantum information science. Next, we will delve into the sources of spectral broadening, including "homogeneous" broadening from dynamical broadening mechanisms in single-particle spectra, heterogeneous broadening from static structural differences in ensemble spectra, and spectral diffusion. Then, we compare the current state of the art in terms of emission line width for a variety of colloidal materials including II-VI quantum dots (QDs) and nanoplatelets, III-V QDs, alloyed QDs, metal-halide perovskites including nanocrystals and 2D structures, doped nanocrystals, and, finally, as a point of comparison, organic molecules. We end with some conclusions and connections, including an outline of promising paths forward. |
| تواريخ الأحداث: | Date Created: 20230613 Date Completed: 20230628 Latest Revision: 20230628 |
| رمز التحديث: | 20230628 |
| DOI: | 10.1021/acs.chemrev.3c00097 |
| PMID: | 37311205 |
| قاعدة البيانات: | MEDLINE |
Find this issue from the American Chemical Society | تدمد: | 1520-6890 |
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| DOI: | 10.1021/acs.chemrev.3c00097 |