دورية أكاديمية

Explainability and human intervention in autonomous scanning probe microscopy.

التفاصيل البيبلوغرافية
العنوان: Explainability and human intervention in autonomous scanning probe microscopy.
المؤلفون: Liu Y; Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 37830, USA., Ziatdinov MA; Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 37830, USA.; Computational Sciences and Engineering Division, Oak Ridge National Laboratory, Oak Ridge, TN 37830, USA., Vasudevan RK; Center for Nanophase Materials Sciences, Oak Ridge National Laboratory, Oak Ridge, TN 37830, USA., Kalinin SV; Department of Materials Science and Engineering, University of Tennessee, Knoxville, TN 37996, USA.
المصدر: Patterns (New York, N.Y.) [Patterns (N Y)] 2023 Oct 09; Vol. 4 (11), pp. 100858. Date of Electronic Publication: 2023 Oct 09 (Print Publication: 2023).
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Elsevier Inc Country of Publication: United States NLM ID: 101767765 Publication Model: eCollection Cited Medium: Internet ISSN: 2666-3899 (Electronic) Linking ISSN: 26663899 NLM ISO Abbreviation: Patterns (N Y) Subsets: PubMed not MEDLINE
أسماء مطبوعة: Original Publication: [New York] : Elsevier Inc., [2020]-
مستخلص: The broad adoption of machine learning (ML)-based autonomous experiments (AEs) in material characterization and synthesis requires strategies development for understanding and intervention in the experimental workflow. Here, we introduce and realize a post-experimental analysis strategy for deep kernel learning-based autonomous scanning probe microscopy. This approach yields real-time and post-experimental indicators for the progression of an active learning process interacting with an experimental system. We further illustrate how this approach can be applied to human-in-the-loop AEs, where human operators make high-level decisions at high latencies setting the policies for AEs, and the ML algorithm performs low-level, fast decisions. The proposed approach is universal and can be extended to other techniques and applications such as combinatorial library analysis.
Competing Interests: The authors declare no conflict of interest.
(© 2023 The Author(s), Oak Ridge National Laboratory.)
References: ACS Nano. 2018 Jun 26;12(6):5185-5189. (PMID: 29790333)
ACS Nano. 2021 Jul 27;15(7):11253-11262. (PMID: 34228427)
Adv Sci (Weinh). 2022 Dec;9(36):e2203422. (PMID: 36344455)
ACS Comb Sci. 2020 Jul 13;22(7):348-355. (PMID: 32551531)
Chem Sci. 2021 Mar 9;12(17):6025-6036. (PMID: 34976336)
J Phys Chem Lett. 2023 Apr 6;14(13):3352-3359. (PMID: 36994975)
Small. 2022 Dec;18(48):e2204130. (PMID: 36253123)
Nanotechnology. 2021 Nov 12;33(5):. (PMID: 34644685)
Patterns (N Y). 2023 Mar 10;4(3):100704. (PMID: 36960442)
Adv Sci (Weinh). 2022 Nov;9(31):e2203957. (PMID: 36065001)
ACS Nano. 2022 Sep 27;16(9):13492-13512. (PMID: 36066996)
Acc Chem Res. 2022 Sep 6;55(17):2454-2466. (PMID: 35948428)
Annu Rev Phys Chem. 2014;65:519-36. (PMID: 24689800)
Sci Adv. 2020 Apr 10;6(15):eaaz1708. (PMID: 32300652)
Adv Mater. 2021 Oct;33(43):e2103680. (PMID: 34510569)
ACS Nano. 2022 Oct 25;16(10):17116-17127. (PMID: 36206357)
ACS Nano. 2022 Jan 25;16(1):1250-1259. (PMID: 34964598)
Chem Sci. 2023 Jan 10;14(6):1443-1452. (PMID: 36794205)
Nanotechnology. 2016 Dec 9;27(49):495703. (PMID: 27827348)
Adv Mater. 2022 May;34(20):e2201345. (PMID: 35279893)
J Am Chem Soc. 2021 Oct 27;143(42):17677-17689. (PMID: 34637304)
Annu Rev Chem Biomol Eng. 2022 Jun 10;13:25-44. (PMID: 35236085)
ACS Nano. 2022 May 24;16(5):7605-7614. (PMID: 35476426)
J Am Chem Soc. 2021 Dec 1;143(47):19945-19955. (PMID: 34793161)
Nanotechnology. 2023 May 22;34(32):. (PMID: 37141868)
فهرسة مساهمة: Keywords: Gaussian process; autonomous experiments; deep kernel learning; human in the loop; scanning probe microscopy
تواريخ الأحداث: Date Created: 20231130 Latest Revision: 20231202
رمز التحديث: 20231202
مُعرف محوري في PubMed: PMC10682748
DOI: 10.1016/j.patter.2023.100858
PMID: 38035198
قاعدة البيانات: MEDLINE
الوصف
تدمد:2666-3899
DOI:10.1016/j.patter.2023.100858