دورية أكاديمية

Porous Tellurium-Doped Ruthenium Dioxide Nanotubes for Enhanced Acidic Water Oxidation.

التفاصيل البيبلوغرافية
العنوان: Porous Tellurium-Doped Ruthenium Dioxide Nanotubes for Enhanced Acidic Water Oxidation.
المؤلفون: Liu GQ; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China., Yang Y; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China., Zhang XL; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China., Li HH; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China., Yu PC; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China., Gao MR; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China., Yu SH; Department of Chemistry, Institute of Biomimetic Materials & Chemistry, New Cornerstone Science Laboratory, Anhui Engineering Laboratory of Biomimetic Materials, Division of Nanomaterials & Chemistry, Hefei National Research Center for Physical Sciences at the Microscale, University of Science and Technology of China, Hefei, 230026, China.
المصدر: Small (Weinheim an der Bergstrasse, Germany) [Small] 2024 Apr; Vol. 20 (16), pp. e2306914. Date of Electronic Publication: 2023 Dec 02.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 101235338 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1613-6829 (Electronic) Linking ISSN: 16136810 NLM ISO Abbreviation: Small Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Original Publication: Weinheim, Germany : Wiley-VCH, c2005-
مستخلص: Electrocatalysts with high activity and durability for acidic oxygen evolution reaction (OER) play a crucial role in achieving cost-effective hydrogen production via proton exchange membrane water electrolysis. A novel electrocatalyst, Te-doped RuO 2 (Te-RuO 2 ) nanotubes, synthesized using a template-directed process, which significantly enhances the OER performance in acidic media is reported. The Te-RuO 2 nanotubes exhibit remarkable OER activity in acidic media, requiring an overpotential of only 171 mV to achieve an anodic current density of 10 mA cm -2 . Furthermore, they maintain stable chronopotentiometric performance under 10 mA cm -2 in acidic media for up to 50 h. Based on the experimental results and density functional calculations, this significant improvement in OER performance to the synergistic effect of large specific surface area and modulated electronic structure resulting from the doping of Te cations is attributed.
(© 2023 Wiley‐VCH GmbH.)
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معلومات مُعتمدة: U1932213 National Natural Science Foundation of China; 22305237 National Natural Science Foundation of China; 21805264 National Natural Science Foundation of China; 2021YFA0715700 National Key Research and Development Program of China; 2018YFE0202201 National Key Research and Development Program of China; New Cornerstone Science Foundation; GXXT-2019-028 University Synergy Innovation Program of Anhui Province; 201903a05020003 Science and Technology Major Project of Anhui Province; 2308085QB39 Natural Science Foundation Youth Project of Anhui Province; 2021TQ0321 China Postdoctoral Science Foundation; 2022M713033 China Postdoctoral Science Foundation; 2022M723032 China Postdoctoral Science Foundation; YD9990002017 USTC Research Funds of the Double First-Class Initiative
فهرسة مساهمة: Keywords: Ru‐based electrocatalyst; acidic water oxidation; electronic structure; oxygen evolution reaction; specific surface area
تواريخ الأحداث: Date Created: 20231202 Latest Revision: 20240418
رمز التحديث: 20240418
DOI: 10.1002/smll.202306914
PMID: 38041488
قاعدة البيانات: MEDLINE
الوصف
تدمد:1613-6829
DOI:10.1002/smll.202306914