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Isotherms, kinetics and thermodynamics of industrial dye acid red 27 adsorption on Sugarcane Bagasse Ash.

التفاصيل البيبلوغرافية
العنوان: Isotherms, kinetics and thermodynamics of industrial dye acid red 27 adsorption on Sugarcane Bagasse Ash.
المؤلفون: de Santana JE; Chemical Engineering Department, Federal University of Pernambuco, Recife, PE, 50.740-590, Brazil. joana.santana@ufpe.br., de Andrade FGS; Chemical Engineering Department, Federal University of Pernambuco, Recife, PE, 50.740-590, Brazil., Ferreira AF; Departament of Fundamental Chemistry, Federal University of Pernambuco, Recife, PE, 50.740-590, Brazil., Ghislandi MG; Engineering Campus, Federal Rural University of Pernambuco, Cabo de Santo Agostinho, PE, 54518-430, Brazil., da Motta Sobrinho MA; Chemical Engineering Department, Federal University of Pernambuco, Recife, PE, 50.740-590, Brazil.
المصدر: Environmental science and pollution research international [Environ Sci Pollut Res Int] 2024 Jan 11. Date of Electronic Publication: 2024 Jan 11.
Publication Model: Ahead of Print
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Springer Country of Publication: Germany NLM ID: 9441769 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1614-7499 (Electronic) Linking ISSN: 09441344 NLM ISO Abbreviation: Environ Sci Pollut Res Int Subsets: MEDLINE
أسماء مطبوعة: Publication: <2013->: Berlin : Springer
Original Publication: Landsberg, Germany : Ecomed
مستخلص: In this study, sugarcane bagasse ash (SCBA), obtained as residue from the sugar mill, was used as an adsorbent for Acid Red 27 (AR27) removal from aqueous solutions. The ash characterization data showed 23.63% of organic compounds and silica (α-SiO 2 ) as the most expressive inorganic compound (confirmed by X-ray diffractogram), the BET surface area had a value of 62.79 m 2 .g -1 and the pH pzc was 8.45. Regarding the adsorptive tests, the optimal initial pH to the dye removal was 2.0. The adsorption equilibrium reached in about 4 h contact time and optimum SCBA dosage was found to be 4 g.L -1 . The pseudo-second order model best represented the adsorption kinetics. The Freundlich equation presented the best fit to the equilibrium data for the removal of AR27 by ash, with maximum adsorption capacity of 15 mg.g -1 at pH 2.0. Thermodynamic study indicate that AR27 adsorption on SCBA occurs through a physisorption mechanism, with ΔHº ads  < 15 kJ.mol -1 . The ΔHº ads evaluated by Vant' Hoff equation was explained as a combination of water desorption enthalpy, ΔHº W and isosteric like enthalpy, ΔHº D for the dye adsorption in liquid environment. The ΔHº D  = 9.2 kJ.mol -1 was calculated from Clausius-Clapeyron approach. The effects of coexisting anions on the adsorption and regeneration and reuse of the adsorbent were also investigated. This study suggests that SCBA, which was used without any pretreatment, has the potential to be applied as a low-cost adsorbent to mitigate effluents contamination with AR27 dye at low concentrations.
(© 2024. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.)
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معلومات مُعتمدة: 142446/2018-1 Conselho Nacional de Desenvolvimento Científico e Tecnológico; BIC-0358-3.07/23 Fundação de Amparo à Ciência e Tecnologia do Estado de Pernambuco
فهرسة مساهمة: Keywords: Adsorption kinetics; Decontamination; Dye adsorption; Isosteric enthalpy; Isotherms; Sugar mill waste; Sustainability
تواريخ الأحداث: Date Created: 20240111 Latest Revision: 20240111
رمز التحديث: 20240111
DOI: 10.1007/s11356-024-31917-x
PMID: 38206467
قاعدة البيانات: MEDLINE
الوصف
تدمد:1614-7499
DOI:10.1007/s11356-024-31917-x