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The Electron Migration Polarization Boosting Electromagnetic Wave Absorption Based on Ce Atoms Modulated yolk@shell Fe x N@NGC.

التفاصيل البيبلوغرافية
العنوان: The Electron Migration Polarization Boosting Electromagnetic Wave Absorption Based on Ce Atoms Modulated yolk@shell Fe x N@NGC.
المؤلفون: Ma Z; Department of Physics, Beijing Technology and Business University, Beijing, 100048, China., Yang K; Department of Physics, Beijing Technology and Business University, Beijing, 100048, China., Li D; School of Science and Engineering, The Chinese University of Hong Kong, Shenzhen, 518172, China., Liu H; School of Chemistry and Chemical Engineering, Xi'an University of Architecture and Technology, Xi'an, 710055, China., Hui S; MOE Key Laboratory of Material Physics and Chemistry under Extraordinary, School of Physical Science and Technology Northwestern Polytechnical University, Xi'an, 710072, China., Jiang Y; Department of Physics, Beijing Technology and Business University, Beijing, 100048, China., Li S; State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing, 102249, China., Li Y; Department of Physics, Beijing Technology and Business University, Beijing, 100048, China., Yang W; State Key Laboratory of Heavy Oil Processing, China University of Petroleum, Beijing, 102249, China., Wu H; MOE Key Laboratory of Material Physics and Chemistry under Extraordinary, School of Physical Science and Technology Northwestern Polytechnical University, Xi'an, 710072, China., Hou Y; Beijing Key Laboratory for Magnetoelectric Materials and Devices, School of Materials Science and Engineering, Peking University, Beijing, 100871, China.; School of Materials, Shenzhen Campus of Sun Yat-Sen University, Shenzhen, 518107, China.
المصدر: Advanced materials (Deerfield Beach, Fla.) [Adv Mater] 2024 Jun; Vol. 36 (23), pp. e2314233. Date of Electronic Publication: 2024 Mar 03.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 9885358 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-4095 (Electronic) Linking ISSN: 09359648 NLM ISO Abbreviation: Adv Mater Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Publication: Sept. 3, 1997- : Weinheim : Wiley-VCH
Original Publication: Deerfield Beach, FL : VCH Publishers, 1989-
مستخلص: The electron migration polarization is considered as a promising approach to optimize electromagnetic waves (EMW) dissipation. However, it is still difficult to realize well-controlled electron migration and elucidate the related EMW loss mechanisms for current researches. Herein, a novel Fe x N@NGC/Ce system to construct an effective electron migration model based on the electron leaps among the 4f/5d/6s orbitals of Ce ions is explored. In Fe 4 N@NGC/Ce SA+Cs+NPs , Ce single-atoms (SA) mainly represent a +3 valence state, which can feed the electrons to Ce 4+ of clusters (Cs) and CeO 2 nanoparticles (NPs) through a conductive network under EMW, leading to the electron migration polarization. Such electron migration loss combined with excellent magnetic loss provided by Fe 4 N core, results in the optimal EMW attenuation performance with a minimum reflection loss exceeds -85.1 dB and a broadened absorption bandwidth up to 7.5 GHz at 1.5 mm. This study clarifies the in-depth relationship between electron migration polarization and EMW dissipation, providing profound insights into developing well-coordinated magnetic-dielectric nanocomposites for EMW absorption engineering.
(© 2024 Wiley‐VCH GmbH.)
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معلومات مُعتمدة: 2022YFA1203902 National Key Research and Development Program of China; 2022YFB3505900 National Key Research and Development Program of China; 92263203 National Natural Science Foundation of China; 52271189 National Natural Science Foundation of China
فهرسة مساهمة: Keywords: Ce single‐atoms; FexN@NGC; electromagnetic wave absorption; electron migration polarization
تواريخ الأحداث: Date Created: 20240221 Latest Revision: 20240607
رمز التحديث: 20240607
DOI: 10.1002/adma.202314233
PMID: 38380795
قاعدة البيانات: MEDLINE
الوصف
تدمد:1521-4095
DOI:10.1002/adma.202314233