دورية أكاديمية

Versatile Titanium Carbide MXene Thin-Film Memristors with Adaptive Learning Behavior.

التفاصيل البيبلوغرافية
العنوان: Versatile Titanium Carbide MXene Thin-Film Memristors with Adaptive Learning Behavior.
المؤلفون: Thomas A; eNDR Laboratory, School of Physics, IISER Thiruvananthapuram, Trivandrum, Kerala 695551, India., Saha P; eNDR Laboratory, School of Physics, IISER Thiruvananthapuram, Trivandrum, Kerala 695551, India., Sahad E M; eNDR Laboratory, School of Physics, IISER Thiruvananthapuram, Trivandrum, Kerala 695551, India., Krishnan K N; eNDR Laboratory, School of Physics, IISER Thiruvananthapuram, Trivandrum, Kerala 695551, India., Das BC; eNDR Laboratory, School of Physics, IISER Thiruvananthapuram, Trivandrum, Kerala 695551, India.
المصدر: ACS applied materials & interfaces [ACS Appl Mater Interfaces] 2024 Apr 09. Date of Electronic Publication: 2024 Apr 09.
Publication Model: Ahead of Print
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: American Chemical Society Country of Publication: United States NLM ID: 101504991 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1944-8252 (Electronic) Linking ISSN: 19448244 NLM ISO Abbreviation: ACS Appl Mater Interfaces Subsets: MEDLINE
أسماء مطبوعة: Original Publication: Washington, D.C. : American Chemical Society
مستخلص: With the advent of the modern era, there is a huge demand for memristor-based neuromorphic computing hardware to overcome the von Neumann bottleneck in traditional computers. Here, we have prepared two-dimensional titanium carbide (Ti 3 C 2 T x ) MXene following the conventional HF etching technique in solution. After confirmation of Ti 3 C 2 T x properties by Raman scattering and crystallinity measurements, high-quality thin-film deposition is realized using an immiscible liquid-liquid interfacial growth technique. Following this, the memristor is fabricated by sandwiching a Ti 3 C 2 T x layer with a thickness of 70 nm between two electrodes. Subsequently, current-voltage ( I-V ) characteristics are measured, revealing a nonvolatile resistive switching property characterized by a swift switching speed of 30 ns and an impressive current On/Off ratio of approximately 10 3 . Furthermore, it exhibits endurance through 500 cycles and retains the states for at least 1 × 10 4 s without observable degradation. Additionally, it maintains a current On/Off ratio of about 10 2 while consuming only femtojoules (fJ) of electrical energy per reading. Systematic I-V results and conductive AFM-based current mapping image analysis are converged to support the electroforming mediated filamentary conduction mechanism. Furthermore, our Ti 3 C 2 T x memristor was found to be truly versatile as an all-in-one device for demonstrating edge computation, logic gate operation, and classical conditioning of learning by the brain in Psychology.
فهرسة مساهمة: Keywords: MXene; classical conditioning; conductive AFM; edge computation; memristor; thin film
تواريخ الأحداث: Date Created: 20240409 Latest Revision: 20240409
رمز التحديث: 20240410
DOI: 10.1021/acsami.3c19177
PMID: 38594622
قاعدة البيانات: MEDLINE
الوصف
تدمد:1944-8252
DOI:10.1021/acsami.3c19177