دورية أكاديمية
Glass-Like Phonon Dynamics and Thermal Transport in a GeTe Nano-Composite at Low Temperature.
العنوان: | Glass-Like Phonon Dynamics and Thermal Transport in a GeTe Nano-Composite at Low Temperature. |
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المؤلفون: | Cravero R; Institute of Light and Matter, UMR5306 Université Lyon 1-CNRS, Université de Lyon, Villeurbanne cedex, F-69622, France.; Institut NEEL, CNRS, Université Grenoble Alpes, 25 avenue des Martyrs, Grenoble, F-38042, France., Tlili A; Institute of Light and Matter, UMR5306 Université Lyon 1-CNRS, Université de Lyon, Villeurbanne cedex, F-69622, France., Paterson J; CEA, LETI, Université Grenoble Alpes, Grenoble, 38000, France., Tomelleri M; CEA, LETI, Université Grenoble Alpes, Grenoble, 38000, France., Marcello P; Institute of Light and Matter, UMR5306 Université Lyon 1-CNRS, Université de Lyon, Villeurbanne cedex, F-69622, France., Debord R; Institute of Light and Matter, UMR5306 Université Lyon 1-CNRS, Université de Lyon, Villeurbanne cedex, F-69622, France., Pailhès S; Institute of Light and Matter, UMR5306 Université Lyon 1-CNRS, Université de Lyon, Villeurbanne cedex, F-69622, France., Bourgeois O; Institut NEEL, CNRS, Université Grenoble Alpes, 25 avenue des Martyrs, Grenoble, F-38042, France., Hippert F; CNRS, Grenoble INP, LMGP, Université Grenoble Alpes, Grenoble, F-38000, France., Le Qui D; FNRS and CESAM, Université de Liége, Sart-Tilman, 4000, Belgique., Raty JY; FNRS and CESAM, Université de Liége, Sart-Tilman, 4000, Belgique., Noe P; CEA, LETI, Université Grenoble Alpes, Grenoble, 38000, France., Giordano VM; Institute of Light and Matter, UMR5306 Université Lyon 1-CNRS, Université de Lyon, Villeurbanne cedex, F-69622, France. |
المصدر: | Small (Weinheim an der Bergstrasse, Germany) [Small] 2024 Jun; Vol. 20 (26), pp. e2310209. Date of Electronic Publication: 2024 Apr 18. |
نوع المنشور: | Journal Article |
اللغة: | English |
بيانات الدورية: | Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 101235338 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1613-6829 (Electronic) Linking ISSN: 16136810 NLM ISO Abbreviation: Small Subsets: PubMed not MEDLINE; MEDLINE |
أسماء مطبوعة: | Original Publication: Weinheim, Germany : Wiley-VCH, c2005- |
مستخلص: | In this work, the experimental evidence of glass-like phonon dynamics and thermal conductivity in a nanocomposite made of GeTe and amorphous carbon is reported, which is of interest for microelectronics, and specifically phase change memories. It is shown that, the total thermal conductivity is reduced by a factor of three at room temperature with respect to pure GeTe, due to the reduction of both electronic and phononic contributions. This latter, similarly to glasses, is small and weakly increasing with temperature between 100 and 300 K, indicating a mostly diffusive thermal transport and reaching a value of 0.86(7) Wm -1 K -1 at room temperature. A thorough investigation of the nanocomposite's phonon dynamics reveals the appearance of an excess intensity in the low energy vibrational density of states, reminiscent of the Boson peak in glasses. These features can be understood in terms of an enhanced phonon scattering at the interfaces, due to the presence of elastic heterogeneities, at wavelengths in the 2-20 nm range. The findings confirm recent simulation results on crystalline/amorphous nanocomposites and open new perspectives in phonon and thermal engineering through the direct manipulation of elastic heterogeneities. (© 2024 The Authors. Small published by Wiley‐VCH GmbH.) |
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معلومات مُعتمدة: | ANR-20-CE05-0046 Agence Nationale de recherche ANR; NanoCHARME AURA - Pack Ambition Recherche |
فهرسة مساهمة: | Keywords: interface; nanocomposite; phonons; thermal conductivity |
تواريخ الأحداث: | Date Created: 20240418 Latest Revision: 20240626 |
رمز التحديث: | 20240627 |
DOI: | 10.1002/smll.202310209 |
PMID: | 38634392 |
قاعدة البيانات: | MEDLINE |
تدمد: | 1613-6829 |
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DOI: | 10.1002/smll.202310209 |