دورية أكاديمية
A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy.
| العنوان: | A US perspective on closing the carbon cycle to defossilize difficult-to-electrify segments of our economy. |
|---|---|
| المؤلفون: | Shaw WJ; Pacific Northwest National Laboratory, Richland, WA, USA. Wendy.shaw@pnnl.gov., Kidder MK; Oak Ridge National Laboratory, Oak Ridge, TN, USA. kidderm@ornl.gov., Bare SR; SLAC National Accelerator Laboratory, Menlo Park, CA, USA. srbare@slac.stanford.edu., Delferro M; Argonne National Laboratory, Lemont, IL, USA. delferro@anl.gov., Morris JR; Ames National Laboratory, Ames, IA, USA. morrisj@ameslab.gov., Toma FM; Lawrence Berkeley National Laboratory, Berkeley, CA, USA. fmtoma@lbl.gov.; Institute of Functional Materials for Sustainability, Helmholtz Zentrum Hereon, Teltow, Brandenburg, Germany. fmtoma@lbl.gov., Senanayake SD; Brookhaven National Laboratory, Upton, NY, USA. ssenanay@bnl.gov., Autrey T; Pacific Northwest National Laboratory, Richland, WA, USA., Biddinger EJ; Department of Chemical Engineering, The City College of New York, New York, NY, USA., Boettcher S; Lawrence Berkeley National Laboratory, Berkeley, CA, USA.; Department of Chemical & Biomolecular Engineering and Department of Chemistry, University of California, Berkeley, Berkeley, CA, USA., Bowden ME; Pacific Northwest National Laboratory, Richland, WA, USA., Britt PF; Oak Ridge National Laboratory, Oak Ridge, TN, USA., Brown RC; Department of Mechanical Engineering, Iowa State University, Ames, IA, USA., Bullock RM; Pacific Northwest National Laboratory, Richland, WA, USA., Chen JG; Brookhaven National Laboratory, Upton, NY, USA.; Department of Chemical Engineering, Columbia University, New York, NY, USA., Daniel C; Argonne National Laboratory, Lemont, IL, USA., Dorhout PK; Vice President for Research, Iowa State University, Ames, IA, USA., Efroymson RA; Oak Ridge National Laboratory, Oak Ridge, TN, USA., Gaffney KJ; SLAC National Accelerator Laboratory, Menlo Park, CA, USA., Gagliardi L; Department of Chemistry, The University of Chicago, Chicago, IL, USA., Harper AS; Pacific Northwest National Laboratory, Richland, WA, USA., Heldebrant DJ; Pacific Northwest National Laboratory, Richland, WA, USA.; Chemical Engineering and Bioengineering, Washington State University, Pullman, WA, USA., Luca OR; Department of Chemistry, University of Colorado Boulder, Boulder, CO, USA., Lyubovsky M; Booz Allen Hamilton, Washington DC, USA., Male JL; Pacific Northwest National Laboratory, Richland, WA, USA.; Biological Systems Engineering Department, Washington State University, Pullman, WA, USA., Miller DJ; Lawrence Berkeley National Laboratory, Berkeley, CA, USA., Prozorov T; Ames National Laboratory, Ames, IA, USA., Rallo R; Pacific Northwest National Laboratory, Richland, WA, USA., Rana R; Department of Chemical Engineering, University of California, Davis, CA, USA., Rioux RM; Department of Chemical Engineering, The Pennsylvania State University, University Park, PA, USA., Sadow AD; Ames National Laboratory, Ames, IA, USA.; Department of Chemistry, Iowa State University, Ames, IA, USA., Schaidle JA; National Renewable Energy Laboratory, Golden, CO, USA., Schulte LA; Department of Natural Resource Ecology and Management, Iowa State University, Ames, IA, USA., Tarpeh WA; Department of Chemical Engineering, Stanford University, Stanford, CA, USA., Vlachos DG; Department of Chemical and Biomolecular Engineering, University of Delaware, Newark, DE, USA., Vogt BD; Department of Chemical Engineering, The Pennsylvania State University, University Park, PA, USA., Weber RS; Pacific Northwest National Laboratory, Richland, WA, USA., Yang JY; Department of Chemistry, University of California Irvine, Irvine, CA, USA., Arenholz E; Pacific Northwest National Laboratory, Richland, WA, USA., Helms BA; Lawrence Berkeley National Laboratory, Berkeley, CA, USA., Huang W; Ames National Laboratory, Ames, IA, USA.; Department of Chemistry, Iowa State University, Ames, IA, USA., Jordahl JL; Department of Natural Resource Ecology and Management, Iowa State University, Ames, IA, USA., Karakaya C; Oak Ridge National Laboratory, Oak Ridge, TN, USA., Kian KC; Independent consultant, Washington DC, USA.; Department of Chemical Engineering, Worcester Polytechnic Institute, Worcester, MA, USA., Kothandaraman J; Pacific Northwest National Laboratory, Richland, WA, USA., Lercher J; Pacific Northwest National Laboratory, Richland, WA, USA.; Department of Chemistry, Technical University of Munich, Munich, Germany., Liu P; Brookhaven National Laboratory, Upton, NY, USA., Malhotra D; Pacific Northwest National Laboratory, Richland, WA, USA., Mueller KT; Pacific Northwest National Laboratory, Richland, WA, USA., O'Brien CP; Department of Chemical and Biomolecular Engineering, University of Notre Dame, Notre Dame, IN, USA., Palomino RM; BASF Corporation, Iselin, NJ, USA., Qi L; Ames National Laboratory, Ames, IA, USA., Rodriguez JA; Brookhaven National Laboratory, Upton, NY, USA., Rousseau R; Oak Ridge National Laboratory, Oak Ridge, TN, USA., Russell JC; Advanced Research Projects Agency - Energy, Department of Energy, Washington DC, USA., Sarazen ML; Department of Chemical and Biological Engineering, Princeton University, Princeton, NJ, USA., Sholl DS; Oak Ridge National Laboratory, Oak Ridge, TN, USA., Smith EA; Ames National Laboratory, Ames, IA, USA.; Department of Chemistry, Iowa State University, Ames, IA, USA., Stevens MB; SLAC National Accelerator Laboratory, Menlo Park, CA, USA., Surendranath Y; Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA, USA., Tassone CJ; SLAC National Accelerator Laboratory, Menlo Park, CA, USA., Tran B; Pacific Northwest National Laboratory, Richland, WA, USA., Tumas W; National Renewable Energy Laboratory, Golden, CO, USA., Walton KS; School of Chemical and Biomolecular Engineering, Georgia Institute of Technology, Atlanta, GA, USA. |
| المصدر: | Nature reviews. Chemistry [Nat Rev Chem] 2024 May; Vol. 8 (5), pp. 376-400. Date of Electronic Publication: 2024 May 01. |
| نوع المنشور: | Journal Article; Review |
| اللغة: | English |
| بيانات الدورية: | Publisher: Springer Nature Country of Publication: England NLM ID: 101703631 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 2397-3358 (Electronic) Linking ISSN: 23973358 NLM ISO Abbreviation: Nat Rev Chem Subsets: PubMed not MEDLINE; MEDLINE |
| أسماء مطبوعة: | Original Publication: [London] : Springer Nature, [2017]- |
| مستخلص: | Electrification to reduce or eliminate greenhouse gas emissions is essential to mitigate climate change. However, a substantial portion of our manufacturing and transportation infrastructure will be difficult to electrify and/or will continue to use carbon as a key component, including areas in aviation, heavy-duty and marine transportation, and the chemical industry. In this Roadmap, we explore how multidisciplinary approaches will enable us to close the carbon cycle and create a circular economy by defossilizing these difficult-to-electrify areas and those that will continue to need carbon. We discuss two approaches for this: developing carbon alternatives and improving our ability to reuse carbon, enabled by separations. Furthermore, we posit that co-design and use-driven fundamental science are essential to reach aggressive greenhouse gas reduction targets. (© 2024. Argonne National Laboratory, Battelle Memorial Institute, UT- Battelle, LLC, Brookhaven National Laboratory, National Renewable Energy Laboratory, AMES National Laboratory, Lawrence Berkley National Laboratory, SLAC National Accelerator Laboratory, Booz Allen Hamilton, BASF Corporation and The Author(s), under exclusive licence to Springer Nature Limited. This work contains contributions, authored by US Government employees in the course of their official duties, which are not subject to copyright protection in the US. Foreign copyright protection for these contributions may still apply.) |
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| DOI: | 10.1038/s41570-024-00587-1 |
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