دورية أكاديمية

Effective Removal of Nile Blue Dye from Wastewater using Silver-Decorated Reduced Graphene Oxide.

التفاصيل البيبلوغرافية
العنوان: Effective Removal of Nile Blue Dye from Wastewater using Silver-Decorated Reduced Graphene Oxide.
المؤلفون: Natasha; Department of Chemistry, Abdul Wali Khan University Mardan, Mardan 23200, Pakistan., Khan A; Department of Chemistry, Abdul Wali Khan University Mardan, Mardan 23200, Pakistan.; Energy, Water and Environment Lab, College of Humanities and Sciences, Prince Sultan University, Riyadh 11586, Saudi Arabia., Rahman UU; Department of Chemistry, Abdul Wali Khan University Mardan, Mardan 23200, Pakistan., Sadaf; Department of Chemistry, Abdul Wali Khan University Mardan, Mardan 23200, Pakistan., Yaseen M; Department of Chemistry, Abdul Wali Khan University Mardan, Mardan 23200, Pakistan., Abumousa RA; Energy, Water and Environment Lab, College of Humanities and Sciences, Prince Sultan University, Riyadh 11586, Saudi Arabia., Khattak R; Department of Chemistry, Shaheed Benazir Bhutto Women University Avenue, Larama Charsadda Road Peshawar, Peshawar 00384,Pakistan., Rehman N; Department of Chemistry, Shaheed Benazir Bhutto University, Sheringal Dir(U), Dir Upper 18000,Pakistan., Bououdina M; Energy, Water and Environment Lab, College of Humanities and Sciences, Prince Sultan University, Riyadh 11586, Saudi Arabia., Humayun M; Energy, Water and Environment Lab, College of Humanities and Sciences, Prince Sultan University, Riyadh 11586, Saudi Arabia.
المصدر: ACS omega [ACS Omega] 2024 Apr 18; Vol. 9 (17), pp. 19461-19480. Date of Electronic Publication: 2024 Apr 18 (Print Publication: 2024).
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: American Chemical Society Country of Publication: United States NLM ID: 101691658 Publication Model: eCollection Cited Medium: Internet ISSN: 2470-1343 (Electronic) Linking ISSN: 24701343 NLM ISO Abbreviation: ACS Omega Subsets: PubMed not MEDLINE
أسماء مطبوعة: Original Publication: Washington, D.C. : American Chemical Society, [2016]-
مستخلص: Nile blue (NB) dye is a highly toxic substance that when discharged into sewage presents a significant risk to the environment and human health. Carbon-based nanomaterials, such as graphene oxide (GO), reduced graphene oxide (rGO), and their nanocomposites, offer considerable potential for eliminating hazardous pollutants from aqueous systems. In this study, we have successfully fabricated bare GO and rGO, and then, the rGO was decorated with silver (Ag) nanoparticles to develop the Ag-rGO composite. The as-prepared materials were characterized by various techniques, such as UV-visible (UV-vis) and Fourier transform infrared (FTIR) spectroscopies, X-ray diffraction (XRD), energy-dispersive X-ray (EDX), and scanning electron microscopy (SEM) to elucidate their structure, morphology, and chemical composition. The pollutant removal performance of the as-prepared materials was evaluated through a batch approach under the effect of various experimental variables for removal of NB dye from wastewater. As obvious, the Ag-rGO composite revealed exceptional performance for NB dye removal from wastewater, with a maximum removal percentage of 94% within 60 min, which is remarkably higher than those of the rGO (i.e., 59%) and GO (i.e., 22%), under the same experimental conditions. The adsorption data was analyzed with thermodynamics, isotherms, and kinetics models to better understand the physicochemical mechanisms driving the effective removal of the NB dye. The results reveal that Ag-rGO nanocomposite exhibit excellent adsorption ability as well as favorable thermodynamic and kinetic parameters for NB dye removal. It was also found that the presence of light enhanced the adsorptive removal of NB while using Ag-rGO as an adsorbent. The present study noted significant reusability of the Ag-rGO nanocomposite, likely due to minimal Ag leaching and/or the robust stability of the Ag-rGO. It is suggested that Ag-rGO-based hybrid materials could serve as promising candidates for efficiently adsorbing and catalytically removing various toxic pollutants from wastewater.
Competing Interests: The authors declare no competing financial interest.
(© 2024 The Authors. Published by American Chemical Society.)
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تواريخ الأحداث: Date Created: 20240506 Latest Revision: 20240507
رمز التحديث: 20240507
مُعرف محوري في PubMed: PMC11064184
DOI: 10.1021/acsomega.4c00973
PMID: 38708276
قاعدة البيانات: MEDLINE
الوصف
تدمد:2470-1343
DOI:10.1021/acsomega.4c00973