دورية أكاديمية
أعرض في EDS

Opening and Constructing Stable Lithium-ion Channels within Polymer Electrolytes.

التفاصيل البيبلوغرافية
العنوان: Opening and Constructing Stable Lithium-ion Channels within Polymer Electrolytes.
المؤلفون: Zhao Y; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Li L; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Zhou D; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Ma Y; School of Materials Science and Engineering, Tianjin University of Technology, Tianjin, 300384, China., Zhang Y; School of Integrative Biological and Chemical Sciences, The University of Texas Rio Grande Valley, Edinburg, TX 78539-2999, USA., Yang H; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Fan S; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Tong H; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Li S; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China., Qu W; School of Materials Science and Chemical Engineering, Harbin University of Science and Technology, Harbin, 150040, China.
المصدر: Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2024 May 17, pp. e202404728. Date of Electronic Publication: 2024 May 17.
Publication Model: Ahead of Print
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 0370543 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-3773 (Electronic) Linking ISSN: 14337851 NLM ISO Abbreviation: Angew Chem Int Ed Engl Subsets: MEDLINE
أسماء مطبوعة: Publication: <2004-> : Weinheim : Wiley-VCH
Original Publication: Weinheim/Bergstr. : New York, : Verlag Chemie ; Academic Press, c1962-
مستخلص: Lithium-ion batteries play an integral role in various aspects of daily life, yet there is a pressing need to enhance their safety and cycling stability. In this study, we have successfully developed a highly secure and flexible solid-state polymer electrolyte (SPE) through the in situ polymerization of allyl acetoacetate (AAA) monomers. This SPE constructed an efficient Li + transport channel inside and effectively improved the solid-solid interface contact of solid-state batteries to reduce interfacial impedance. Furthermore, it exhibited excellent thermal stability, an ionic conductivity of 3.82×10 -4  S cm -1 at room temperature (RT), and a Li + transport number (t Li+ ) of 0.66. The numerous oxygen vacancies on layered inorganic SiO 2 created an excellent environment for TFSI - immobilization. Free Li + migrated rapidly at the C=O equivalence site with the poly(allyl acetoacetate) (PAAA) matrix. Consequently, when cycled at 0.5C and RT, it displayed an initial discharge specific capacity of 140.6 mAh g -1 with a discharge specific capacity retention rate of 70 % even after 500 cycles. Similarly, when cycled at a higher rate of 5C, it demonstrated an initial discharge specific capacity of 132.3 mAh g -1 while maintaining excellent cycling stability.
(© 2024 Wiley-VCH GmbH.)
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معلومات مُعتمدة: 2022CXRCCG007 the Harbin Manufacturing Science and Technology Innovation Talent Project; HST2022DQ007 Heilongjiang Province Ecological Environment Protection Research Project; 21706043 National Natural Science Foundation of China
فهرسة مساهمة: Keywords: facilitate lithium-ion migration; in situ construction; lithium-ion batteries; lithium-ion channel; solid-state polymer electrolyte
تواريخ الأحداث: Date Created: 20240518 Latest Revision: 20240626
رمز التحديث: 20240626
DOI: 10.1002/anie.202404728
PMID: 38760998
قاعدة البيانات: MEDLINE
الوصف
تدمد:1521-3773
DOI:10.1002/anie.202404728