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Photochargeable Mn-Based Metal-Organic Framework and Decoupled Photocatalysis.

التفاصيل البيبلوغرافية
العنوان: Photochargeable Mn-Based Metal-Organic Framework and Decoupled Photocatalysis.
المؤلفون: Wu S; Chair of Inorganic and Metal-Organic Chemistry, Department of Chemistry, and Catalysis Research Center (CRC), TUM School of Natural Sciences, Technical University of Munich, Garching, Germany., Stanley PM; Chair of Inorganic and Metal-Organic Chemistry, Department of Chemistry, and Catalysis Research Center (CRC), TUM School of Natural Sciences, Technical University of Munich, Garching, Germany., Deger SN; Chair of Inorganic and Metal-Organic Chemistry, Department of Chemistry, and Catalysis Research Center (CRC), TUM School of Natural Sciences, Technical University of Munich, Garching, Germany., Hussain MZ; Chair of Inorganic and Metal-Organic Chemistry, Department of Chemistry, and Catalysis Research Center (CRC), TUM School of Natural Sciences, Technical University of Munich, Garching, Germany., Jentys A; Chair of Industrial Chemistry and Heterogenous Catalysis, Department of Chemistry, and Catalysis Research Center (CRC), TUM School of Natural Sciences, Technical University of Munich, Garching, Germany., Warnan J; Chair of Inorganic and Metal-Organic Chemistry, Department of Chemistry, and Catalysis Research Center (CRC), TUM School of Natural Sciences, Technical University of Munich, Garching, Germany.
المصدر: Angewandte Chemie (International ed. in English) [Angew Chem Int Ed Engl] 2024 Sep 09; Vol. 63 (37), pp. e202406385. Date of Electronic Publication: 2024 Jul 29.
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 0370543 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1521-3773 (Electronic) Linking ISSN: 14337851 NLM ISO Abbreviation: Angew Chem Int Ed Engl Subsets: PubMed not MEDLINE; MEDLINE
أسماء مطبوعة: Publication: <2004-> : Weinheim : Wiley-VCH
Original Publication: Weinheim/Bergstr. : New York, : Verlag Chemie ; Academic Press, c1962-
مستخلص: Designing multifunctional materials that mimic the light-dark decoupling of natural photosynthesis is a key challenge in the field of energy conversion. Herein, we introduce MnBr-253, a precious metal-free metal-organic framework (MOF) built on Al nodes, bipyridine linkers and MnBr(CO) 3 (bipyridine) complexes. Upon irradiation, MnBr-253 colloids demonstrate an electron photocharging capacity of ~42 C ⋅ g -1 MOF , with state-of-the-art photocharging rate (1.28 C ⋅ s -1  ⋅ g -1 MOF ) and incident photon-to-electron conversion efficiency of ~9.4 % at 450 nm. Spectroscopic and computational studies support effective electron accumulation at the Mn complex while high porosity and Mn loading account for the notable electron storage performance. The charged MnBr-253 powders were successfully applied for hydrogen evolution under dark conditions thus emulating the light-decoupled reactivity of photosynthesis.
(© 2024 The Author(s). Angewandte Chemie International Edition published by Wiley-VCH GmbH.)
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معلومات مُعتمدة: Excellence Cluster 2089 "e-conversion" Deutsche Forschungsgemeinschaft; 451579122 Deutsche Forschungsgemeinschaft; Chinese Government Scholarship
فهرسة مساهمة: Keywords: Dark Photocatalysis; Electron accumulation; Metal–Organic Framework; Mn complex; Photocharging
تواريخ الأحداث: Date Created: 20240729 Latest Revision: 20240902
رمز التحديث: 20240902
DOI: 10.1002/anie.202406385
PMID: 39074974
قاعدة البيانات: MEDLINE
الوصف
تدمد:1521-3773
DOI:10.1002/anie.202406385