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Droplet Friction on Superhydrophobic Surfaces Scales With Liquid-Solid Contact Fraction.

التفاصيل البيبلوغرافية
العنوان: Droplet Friction on Superhydrophobic Surfaces Scales With Liquid-Solid Contact Fraction.
المؤلفون: Lepikko S; Department of Applied Physics, Aalto University, P.O. Box 15600, Espoo, 02150, Finland.; Center of Excellence in Life-Inspired Hybrid Materials (LIBER), Aalto University, P.O. Box 15600, Espoo, 02150, Finland., Turkki V; Department of Applied Physics, Aalto University, P.O. Box 15600, Espoo, 02150, Finland.; Center of Excellence in Life-Inspired Hybrid Materials (LIBER), Aalto University, P.O. Box 15600, Espoo, 02150, Finland., Koskinen T; Department of Electronics and Nanoengineering, Aalto University, P.O. Box 13500, Espoo, 02150, Finland., Raju R; Department of Electronics and Nanoengineering, Aalto University, P.O. Box 13500, Espoo, 02150, Finland., Jokinen V; Department of Chemistry and Materials Science, Aalto University, P.O. Box 16100, Espoo, 02150, Finland., Kiseleva MS; Department of Applied Physics, Aalto University, P.O. Box 15600, Espoo, 02150, Finland.; Center of Excellence in Life-Inspired Hybrid Materials (LIBER), Aalto University, P.O. Box 15600, Espoo, 02150, Finland., Rantataro S; Department of Electrical Engineering and Automation, Aalto University, Maarintie 8, Espoo, 02150, Finland., Timonen JVI; Department of Applied Physics, Aalto University, P.O. Box 15600, Espoo, 02150, Finland.; Center of Excellence in Life-Inspired Hybrid Materials (LIBER), Aalto University, P.O. Box 15600, Espoo, 02150, Finland., Backholm M; Department of Applied Physics, Aalto University, P.O. Box 15600, Espoo, 02150, Finland.; Center of Excellence in Life-Inspired Hybrid Materials (LIBER), Aalto University, P.O. Box 15600, Espoo, 02150, Finland., Tittonen I; Department of Electronics and Nanoengineering, Aalto University, P.O. Box 13500, Espoo, 02150, Finland., Ras RHA; Department of Applied Physics, Aalto University, P.O. Box 15600, Espoo, 02150, Finland.; Center of Excellence in Life-Inspired Hybrid Materials (LIBER), Aalto University, P.O. Box 15600, Espoo, 02150, Finland.
المصدر: Small (Weinheim an der Bergstrasse, Germany) [Small] 2024 Sep 17, pp. e2405335. Date of Electronic Publication: 2024 Sep 17.
Publication Model: Ahead of Print
نوع المنشور: Journal Article
اللغة: English
بيانات الدورية: Publisher: Wiley-VCH Country of Publication: Germany NLM ID: 101235338 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1613-6829 (Electronic) Linking ISSN: 16136810 NLM ISO Abbreviation: Small Subsets: MEDLINE
أسماء مطبوعة: Original Publication: Weinheim, Germany : Wiley-VCH, c2005-
مستخلص: It is generally assumed that contact angle hysteresis of superhydrophobic surfaces scales with liquid-solid contact fraction, however, its experimental verification has been problematic due to the limited accuracy of contact angle and sliding angle goniometry. Advances in cantilever-based friction probes enable accurate droplet friction measurements down to the nanonewton regime, thus suiting much better for characterizing the wetting of superhydrophobic surfaces than contact angle hysteresis measurements. This work quantifies the relationship between droplet friction and liquid-solid contact fraction, through theory and experimental validation. Well-defined micropillar and microcone structures are used as model surfaces to provide a wide range of different liquid-solid contact fractions. Micropillars are known to be able to hold the water on top of them, and a theoretical analysis together with confocal laser scanning microscopy shows that despite the spiky nature of the microcones droplets do not sink into the conical structure either, rendering a diminishingly small liquid-solid contact fraction. Droplet friction characterization with a micropipette force sensor technique reveals a strong dependence of the droplet friction on the contact fraction, and the dependency is described with a simple physical equation, despite the nearly three-orders-of-magnitude difference in liquid-solid contact fraction between the sparsest cone surface and the densest pillar surface.
(© 2024 The Author(s). Small published by Wiley‐VCH GmbH.)
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معلومات مُعتمدة: International ERC_ European Research Council; Center of Excellence Programme; 346109 Life-Inspired Hybrid Materials (LIBER); 346112 Life-Inspired Hybrid Materials (LIBER); 725513 Consolidator Grant SuperRepel; Tandem Industry Academia; Project No. 239 Finnish Research Impact Foundation; 341459 Academy of Finland; 309237 Academy of Finland; 329406 Academy of Finland
فهرسة مساهمة: Keywords: contact angle hysteresis; droplet friction; liquid–solid contact fraction; superhydrophobicity
تواريخ الأحداث: Date Created: 20240917 Latest Revision: 20240917
رمز التحديث: 20240918
DOI: 10.1002/smll.202405335
PMID: 39286993
قاعدة البيانات: MEDLINE
الوصف
تدمد:1613-6829
DOI:10.1002/smll.202405335