التفاصيل البيبلوغرافية
| العنوان: |
Metal-related electrocatalysts for Li–CO2 batteries: an overview of the fundamentals to explore future-oriented strategies. |
| المؤلفون: |
Lv, Huanzhu, Huang, Xiang Long, Zhu, Xiaoqi, Wang, Bin |
| المصدر: |
Journal of Materials Chemistry A; 12/28/2022, Vol. 10 Issue 48, p25406-25430, 25p |
| مستخلص: |
In the context of carbon peaking and carbon neutrality, the recovery and utilization of clean CO2 in energy storage systems have attracted significant attention from researchers. Recently, Li–CO2 batteries, that utilize CO2 as the cathode material, have been proposed to improve the economics of CO2 capture and reduce the accumulation of CO2, which can be applied to address problems with the operating environment. However, as an emerging research direction, this Li–CO2 battery system still faces many difficulties that require to be overcome, such as poor reversibility, low energy efficiency, and high overpotential, which are caused by poor electrochemical reaction kinetics. Therefore, designing and developing catalysts for Li–CO2 batteries with excellent catalytic activity and stability is pivotal in settling the above problems. In this review, the reduction and oxidation mechanisms of Li–O2/CO2 and Li–CO2 batteries are introduced first. Next, a comprehensive and exhaustive review is provided to discuss the cutting-edge design strategies of materials and structures of metal-based electrocatalysts oriented by Li–CO2 batteries. Finally, based on the research progress of advanced Li–CO2 batteries in the past few years, the opportunities and challenges for the future development of Li–CO2 batteries are highlighted. [ABSTRACT FROM AUTHOR] |
|
Copyright of Journal of Materials Chemistry A is the property of Royal Society of Chemistry and its content may not be copied or emailed to multiple sites or posted to a listserv without the copyright holder's express written permission. However, users may print, download, or email articles for individual use. This abstract may be abridged. No warranty is given about the accuracy of the copy. Users should refer to the original published version of the material for the full abstract. (Copyright applies to all Abstracts.) |
| قاعدة البيانات: |
Complementary Index |
