التفاصيل البيبلوغرافية
| العنوان: |
MOF 基单原子催化剂用于 CO2 还原的研究进展. (Chinese) |
| Alternate Title: |
Research Progress on MOF-based Single-atom Catalysts for CO2 Reduction. (English) |
| المؤلفون: |
贾宇桐, 周阿武, 赵 琛, 张 岩, 张更新, 谢亚勃, 李建荣 |
| المصدر: |
Journal of Beijing University of Technology; Feb2024, Vol. 50 Issue 2, p216-229, 14p |
| Abstract (English): |
Utilization of CO2 into value-added products is one of the important ways to achieve carbon neutrality. Metal-organic frameworks (MOF) have been proven to be promising and effective materials, relying on the characteristic of porosity, functional adjustability, abundant active sites and high specific surface area. Single-atom catalysts (SAC) have emerged as a new frontier due to well-defined structures and maximum atom utilization efficiency (100% ). By combining the merits of both, MOF-based SAC exhibits enormous potential in photocatalytic / electrocatalytic CO2 reduction reactions. The review systematically summarized the latest research progress of MOF-based SAC in photocatalytic /electrocatalytic CO2 reduction. The diverse fabrication strategies and principles of MOF-based SAC, including MOF-immobilized SAC and MOF-derived SAC, as well as unique advantages demonstrated in photocatalytic / electrocatalytic CO2 reduction, were discussed. Finally, a perspective on MOF- photocatalysts/ electrocatalysts for CO2 reduction was given. [ABSTRACT FROM AUTHOR] |
| Abstract (Chinese): |
CO2资源化利用是实现“双碳冶目标的重要途径之一. 金属有机框架(metal鄄organic frameworks, MOF)材料 具有高孔隙率、可调节的功能、丰富的活性位点和潜在锚定位点等优点;单原子催化剂( single鄄atom catalysts, SAC) 有独特的电子结构和最大化金属利用率的优点. 结合二者的优势, MOF 基单原子催化剂在光/ 电催化 CO2还原反 应中表现出良好的应用前景. 系统地总结了 MOF 基单原子催化剂在光/ 电催化 CO2还原中的最新研究进展, 主要 分为 2 个部分:纯 MOF 固定的 SAC 和 MOF 衍生的 SAC, 分别探讨了各种制备策略和原理及在光/ 电催化 CO2还原 中展现的独特优势, 并从理化特性上分析了材料性能优势的成因. 最后对以 MOF 基材料为光/ 电催化 CO2还原催 化剂的研究进行了总结和展望. [ABSTRACT FROM AUTHOR] |
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| قاعدة البيانات: |
Complementary Index |
