High-Resolution Gamma Spectrometry of a Plutonium Bearing Waste Drum With High-Energy Reaction-Induced Gamma Rays

التفاصيل البيبلوغرافية
العنوان: High-Resolution Gamma Spectrometry of a Plutonium Bearing Waste Drum With High-Energy Reaction-Induced Gamma Rays
المؤلفون: G. Faussier, P. G. Allinei, R. De Stefano, V. Bottau, L. Tondut, C. Carasco, Cyrille Eleon, Bertrand Perot
المصدر: IEEE Transactions on Nuclear Science. 67:575-584
بيانات النشر: Institute of Electrical and Electronics Engineers (IEEE), 2020.
سنة النشر: 2020
مصطلحات موضوعية: Physics, Nuclear and High Energy Physics, Physics::Instrumentation and Detectors, 010308 nuclear & particles physics, Astrophysics::High Energy Astrophysical Phenomena, Gamma ray, Radioactive waste, chemistry.chemical_element, Scintillator, Inelastic scattering, 01 natural sciences, Neutron temperature, Plutonium, Nuclear physics, Nuclear Energy and Engineering, chemistry, 0103 physical sciences, Neutron, Coincidence counting, Electrical and Electronic Engineering
الوصف: In the framework of the radioactive waste drum characterization using neutron coincidence counting, the Nuclear Measurement Laboratory of French Alternative Energies and Atomic Energy Commission (CEA) Cadarache is studying plastic scintillators as an alternative to ideal but costly 3He gas proportional counters. Plastic scintillators are at least five times cheaper for the same detection efficiency, and in addition, they detect fast neutrons three orders of magnitude more quickly than 3He detectors. However, they are sensitive to gamma rays with no pulse shape discrimination abilities for large detection volumes, which implies the necessity to identify precisely gamma background sources that may affect the useful signal. This article presents a detailed analysis of the gamma-ray spectrum of a radioactive waste drum containing glove box filters contaminated by plutonium dioxide. Classical gamma emissions following alpha and beta disintegrations are identified, and also those accompanying inelastic scattering (n, $\text{n}^{\prime }$ ) or radiative capture (n, $\gamma$ ) reactions in the whole waste drum, and ( $\alpha $ , n) or ( $\alpha $ , p) reactions in the filtration media, which can lead to neutron-gamma coincidences parasitizing useful coincidences from plutonium spontaneous fissions.
تدمد: 1558-1578
0018-9499
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::1b8af351cd4d83fffac60d9509d11e30
https://doi.org/10.1109/tns.2019.2959079
حقوق: OPEN
رقم الأكسشن: edsair.doi...........1b8af351cd4d83fffac60d9509d11e30
قاعدة البيانات: OpenAIRE