Temperature dependence of dissolution rate of a lead oxide mass exchanger in lead–bismuth eutectic

التفاصيل البيبلوغرافية
العنوان: Temperature dependence of dissolution rate of a lead oxide mass exchanger in lead–bismuth eutectic
المؤلفون: Alessandro Marino, J. Lim, J. Van den Bosch, Stuart A. Maloy, Keith Albert Woloshun, F. Rubio, M. Caro, J. Deconinck, S. Keijers
المصدر: Journal of Nuclear Materials. 450:270-277
بيانات النشر: Elsevier BV, 2014.
سنة النشر: 2014
مصطلحات موضوعية: Packed bed, Nuclear and High Energy Physics, Lead-bismuth eutectic, Chemistry, Inorganic chemistry, Thermodynamics, Reynolds number, Sherwood number, Boundary layer, symbols.namesake, Nuclear Energy and Engineering, symbols, General Materials Science, Limiting oxygen concentration, Dissolution, Lead oxide
الوصف: A Computational Fluid Dynamic (CFD) model of a lead oxide mass exchanger (PbO MX) was developed. The mass exchanger consisted of a packed bed of PbO spheres. The geometry was created using Discrete Elements Method (DEM) software while the meshing, the solving and the post-processing were done by the commercial CFD package CFX. The dissolution process was modeled by implementing in the code oxygen mass transfer through the boundary layer. The dissolution rate was then predicted for different temperatures. Experiments were also performed at the LBE material test loop known as the DELTA loop. Oxygen concentration at the outlet of the PbO MX was measured for different conditions using a potentiometric oxygen sensor and the dissolution rate was determined for five different temperatures. The experimental data were compared with the numerical model. The temperature dependence of the dissolution rate was then determined in terms of Sherwood number by fitting the simulation results while keeping constant Reynolds number. The results showed that the Sherwood number for PbO MX in flowing LBE varies with Sc 0.323 .
تدمد: 0022-3115
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::72f3b1ba3fd095a27b5b5ad22f2a59ef
https://doi.org/10.1016/j.jnucmat.2013.12.023
رقم الأكسشن: edsair.doi...........72f3b1ba3fd095a27b5b5ad22f2a59ef
قاعدة البيانات: OpenAIRE