Ferromagnetism in van der Waals compound MnSb1.8Bi0.2Te4

التفاصيل البيبلوغرافية
العنوان: Ferromagnetism in van der Waals compound MnSb1.8Bi0.2Te4
المؤلفون: Julie A. Borchers, Ke Wang, Zhiqiang Mao, Colin Heikes, Yingdong Guan, Yu Wang, Paweł Zajdel, Jun Zhu, Seng Huat Lee, Yanglin Zhu, Patrick Quarterman, William Ratcliff, Yangyang Chen, Ya Wen Chuang, Kevin Honz
المصدر: Physical Review Materials. 4
بيانات النشر: American Physical Society (APS), 2020.
سنة النشر: 2020
مصطلحات موضوعية: Materials science, Physics and Astronomy (miscellaneous), Magnetism, Order (ring theory), 02 engineering and technology, 021001 nanoscience & nanotechnology, Coupling (probability), 01 natural sciences, Magnetization, Crystallography, Ferromagnetism, 0103 physical sciences, Antiferromagnetism, Curie temperature, General Materials Science, 010306 general physics, 0210 nano-technology, Ground state
الوصف: The intersection of topology and magnetism represents a new playground to discover novel quantum phenomena and device concepts. In this work, we show that under certain synthetic conditions, a van der Waals single-crystalline compound $\mathrm{MnS}{\mathrm{b}}_{1.8}\mathrm{B}{\mathrm{i}}_{0.2}\mathrm{T}{\mathrm{e}}_{4}$ exhibits a net ferromagnetic state with a Curie temperature of 26 K, in contrast to the fully compensated antiferromagnetic order observed previously for other members of the $\mathrm{Mn}{(\mathrm{Sb},\mathrm{Bi})}_{2}\mathrm{T}{\mathrm{e}}_{4}$ family. We employ magneto-transport, bulk magnetization, x-ray and neutron scattering studies to illustrate the structural, magnetic, and electrical properties of $\mathrm{MnS}{\mathrm{b}}_{1.8}\mathrm{B}{\mathrm{i}}_{0.2}\mathrm{T}{\mathrm{e}}_{4}$. Our structural analyses reveal considerable Mn-Sb site mixing and suggest a recently proposed mechanism, where Mn occupying the Sb site mediates a ferromagnetic coupling between Mn layers [Murakami et al., Phys. Rev. B 100, 195103 (2019)], could be at play. Close comparisons made to an antiferromagnetic compound $\mathrm{MnS}{\mathrm{b}}_{2}\mathrm{T}{\mathrm{e}}_{4}$ illustrate the subtle magnetic interactions of the system and the important role played by local chemistry. The appearance of an unusual anomalous Hall effect in $\mathrm{MnS}{\mathrm{b}}_{1.8}\mathrm{B}{\mathrm{i}}_{0.2}\mathrm{T}{\mathrm{e}}_{4}$ at low temperatures hints at a magnetic ground state different from other members of this family. Our results are an important step in the synthesis and understanding of magnetism in materials with topological characteristics.
تدمد: 2475-9953
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::f9679cb4a6c386816fe5cfef0b22f342
https://doi.org/10.1103/physrevmaterials.4.064411
حقوق: OPEN
رقم الأكسشن: edsair.doi...........f9679cb4a6c386816fe5cfef0b22f342
قاعدة البيانات: OpenAIRE