Geochemistry of PM10 over Europe during the EMEP intensive measurement periods in summer 2012 and winter 2013

التفاصيل البيبلوغرافية
العنوان: Geochemistry of PM10 over Europe during the EMEP intensive measurement periods in summer 2012 and winter 2013
المؤلفون: Andrés Alastuey, Xavier Querol, Wenche Aas, Franco Lucarelli, Noemí Perez, Teresa Moreno, Fabrizia Cavalli, Hans Areskoug, Violeta Balan, Maria Catrambone, Darius Ceburnis, José C. Cerro, Sébastien Conil, Lusine Gevorgyan, Christoph Hueglin, Kornelia Imre, Jean-Luc Jafrezzo, Sarah R. Leeson, Nikolaos Mihalopoulos, Marta Mitosinkova, Jorge Pey, Jean-Philippe Putaud, Véronique Riffault, Anna Ripoll, Jean Sciare, Karine Sellegri, Gerald Spinder, Karl Espen Yttri
بيانات النشر: Copernicus GmbH, 2016.
سنة النشر: 2016
مصطلحات موضوعية: complex mixtures
الوصف: Abstract. The third intensive measurement period (IMP) organised by the European Monitoring and Evaluation Programme (EMEP) under the UNECE CLTRAP took place in summer 2012 and winter 2013, with PM10 filter samples concurrently collected at 20 (16 EMEP) regional background sites across Europe for subsequent analysis of their mineral dust content. All samples were analysed by the same or a comparable methodology. Higher PM10 mineral dust loadings were observed at most sites in summer (0.5–10 µg m−3) compared to winter (0.2–2 µg m−3), with the most elevated concentrations in the southern- and easternmost countries, accounting for 20–40 % of PM10. Saharan dust outbreaks were responsible for the high summer dust loadings at western and central European sites, whereas regional or local sources explained the elevated concentrations observed at eastern sites. The eastern Mediterranean sites experienced elevated levels due to African dust outbreaks during both summer and winter. The mineral dust composition varied more in winter than in summer, with a higher relative contribution of anthropogenic dust during the former period. A relatively high contribution of K from non-mineral and non-seasalt sources, such as biomass burning, was evident in winter at some of the central and eastern European sites. The spatial distribution of some components and metals reveals the influence of specific anthropogenic sources on a regional scale: shipping emissions (V, Ni, and SO42−) in the Mediterranean region, metallurgy (Cr, Ni, and Mn) in Central and Eastern Europe, coal combustion (As, Se, and SO42−) in Eastern countries, and traffic (Cu) at sites affected by emissions from nearby cities.
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_________::fc87d74507211d8b31114686e9e3cda9
https://doi.org/10.5194/acp-2016-42
حقوق: OPEN
رقم الأكسشن: edsair.doi...........fc87d74507211d8b31114686e9e3cda9
قاعدة البيانات: OpenAIRE