Airborne mercury species at the Råö background monitoring site in Sweden: distribution of mercury as an effect of long-range transport

التفاصيل البيبلوغرافية
العنوان: Airborne mercury species at the Råö background monitoring site in Sweden: distribution of mercury as an effect of long-range transport
المؤلفون: John Munthe, Katarina Gårdfeldt, Michelle G. Nerentorp Mastromonaco, Ingvar Wängberg
المصدر: Atmospheric Chemistry and Physics, Vol 16, Pp 13379-13387 (2016)
بيانات النشر: Copernicus GmbH, 2016.
سنة النشر: 2016
مصطلحات موضوعية: Atmospheric Science, Ozone, 010504 meteorology & atmospheric sciences, Meteorology, chemistry.chemical_element, Elemental mercury, 010501 environmental sciences, Particulates, Atmospheric sciences, 01 natural sciences, Monitoring site, lcsh:QC1-999, Mercury (element), lcsh:Chemistry, Troposphere, chemistry.chemical_compound, Observation system, lcsh:QD1-999, chemistry, Environmental science, Annual variation, lcsh:Physics, 0105 earth and related environmental sciences
الوصف: Within the EU-funded project, Global Mercury Observation System (GMOS) airborne mercury has been monitored at the background Råö measurement site on the western coast of Sweden from mid-May 2012 to the beginning of July 2013 and from the beginning of February 2014 to the end of May 2015. The following mercury species/fractions were measured: gaseous elemental mercury (GEM), particulate bound mercury (PBM) and gaseous oxidised mercury (GOM) using the Tekran measurement system. The mercury concentrations measured at the Råö site were found to be low in comparison to other, comparable, European measurement sites. A back-trajectory analysis to study the origin of air masses reaching the Råö site was performed. Due to the remote location of the Råö measurement station it receives background air about 60 % of the time. However, elevated mercury concentrations arriving with air masses coming from the south-east are noticeable. GEM and PBM concentrations show a clear annual variation with the highest values occurring during winter, whereas the highest concentrations of GOM were obtained in spring and summer. An evaluation of the diurnal pattern of GOM, with peak concentrations at midday or in the early afternoon, which often is observed at remote places, shows that it is likely to be driven by local meteorology in a similar way to ozone. Evidence that a significant part of the GOM measured at the Råö site has been formed in free tropospheric air is presented.
تدمد: 1680-7324
URL الوصول: https://explore.openaire.eu/search/publication?articleId=doi_dedup___::0b0817e483e4f9ac5e49e831f18d9f7c
https://doi.org/10.5194/acp-16-13379-2016
حقوق: OPEN
رقم الأكسشن: edsair.doi.dedup.....0b0817e483e4f9ac5e49e831f18d9f7c
قاعدة البيانات: OpenAIRE